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Dynamic properties of spin cluster glass and the exchange bias effect in BiFeO3 nanocrystals
Dong, Sining1; Yao, Yiping1; Hou, Ying1; Liu, Yukuai1; Tang, Yang1; Li, Xiaoguang1,2
通讯作者Li, Xiaoguang(lixg@ustc.edu.cn)
2011-09-23
发表期刊NANOTECHNOLOGY
ISSN0957-4484
卷号22期号:38页码:8
摘要A spin cluster glass behavior and a complicated exchange bias effect are observed in high quality BiFeO3 nanocrystals grown by a hydrothermal method. The dynamic properties of the spin clusters investigated by measuring the frequency dependences of ac susceptibility show that the relaxation process can be described using a power law with the glass transition temperature T-g = 57 K, relaxation time constant tau(0) = 4.4 x 10(-10) s, and critical exponent zv = 10.3 +/- 1.9, consistent with a three-dimensional Ising spin glass. The exchange bias field (H-EB) varies non-monotonically with temperature and achieves a minimum at T-g. The abnormal shift of hysteresis loops above T-g may be interpreted in terms of a Malozemoff's random-field model with a framework of antiferromagnetic core/spin-cluster shell structure and a two-dimensional diluted antiferromagnet in a field (2D-DAFF) model, respectively. The exchange anisotropy of the BiFeO3 nanocrystals will shed light on a possible application for magnetism related nanosized devices.
资助者National Natural Science Foundation of China ; National Basic Research Program of China
DOI10.1088/0957-4484/22/38/385701
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China ; National Basic Research Program of China[2011CBA00102] ; National Basic Research Program of China[2009CB929502]
WOS研究方向Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号WOS:000294722400008
出版者IOP PUBLISHING LTD
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被引频次:63[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/105367
专题中国科学院金属研究所
通讯作者Li, Xiaoguang
作者单位1.Univ Sci & Technol China, Dept Phys, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China
2.Acad Sinica, Int Ctr Mat Phys, Shenyang 110015, Peoples R China
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Dong, Sining,Yao, Yiping,Hou, Ying,et al. Dynamic properties of spin cluster glass and the exchange bias effect in BiFeO3 nanocrystals[J]. NANOTECHNOLOGY,2011,22(38):8.
APA Dong, Sining,Yao, Yiping,Hou, Ying,Liu, Yukuai,Tang, Yang,&Li, Xiaoguang.(2011).Dynamic properties of spin cluster glass and the exchange bias effect in BiFeO3 nanocrystals.NANOTECHNOLOGY,22(38),8.
MLA Dong, Sining,et al."Dynamic properties of spin cluster glass and the exchange bias effect in BiFeO3 nanocrystals".NANOTECHNOLOGY 22.38(2011):8.
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