Seebeck coefficient of Ln (x) Ca1-x MnO3 perovskites in paramagnetic state | |
Wang, Yang1,2; Sui, Yu2,3; Wang, Xianjie2; Su, Wenhui2,3 | |
通讯作者 | Wang, Yang(wang_yang@ntu.edu.sg) |
2011-07-01 | |
发表期刊 | APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING
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ISSN | 0947-8396 |
卷号 | 104期号:1页码:135-142 |
摘要 | The Seebeck coefficient is a function of carrier concentration and configurational entropy. In this report, we semi-theoretically investigate the Seebeck coefficient of Ln (x) Ca1-x MnO3 (Ln=Rare-earth) perovskites based on the electronic structure of the 3d orbitals of Mn ions, using the developed Heikes model, Boltzmann transport model, and diffusion model. The results show that the Seebeck coefficient of such a strongly correlated electron system in paramagnetic state is remarkably affected by site degeneracy. As temperature decreases, the evolution of the spin and orbital degrees of freedom together with the change in phonon scattering mode describes the Seebeck coefficient behavior satisfactorily. The phonon drag effect at low temperature is also discussed. |
资助者 | National Natural Science Foundation of China |
DOI | 10.1007/s00339-010-6081-6 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China[50672019] ; National Natural Science Foundation of China[10804024] |
WOS研究方向 | Materials Science ; Physics |
WOS类目 | Materials Science, Multidisciplinary ; Physics, Applied |
WOS记录号 | WOS:000291652600020 |
出版者 | SPRINGER |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/106492 |
专题 | 中国科学院金属研究所 |
通讯作者 | Wang, Yang |
作者单位 | 1.Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore 2.Harbin Inst Technol, Ctr Condensed Matter Sci & Technol CCMST, Dept Phys, Harbin 150001, Peoples R China 3.Acad Sinica, Int Ctr Mat Phys, Shenyang 110015, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Yang,Sui, Yu,Wang, Xianjie,et al. Seebeck coefficient of Ln (x) Ca1-x MnO3 perovskites in paramagnetic state[J]. APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING,2011,104(1):135-142. |
APA | Wang, Yang,Sui, Yu,Wang, Xianjie,&Su, Wenhui.(2011).Seebeck coefficient of Ln (x) Ca1-x MnO3 perovskites in paramagnetic state.APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING,104(1),135-142. |
MLA | Wang, Yang,et al."Seebeck coefficient of Ln (x) Ca1-x MnO3 perovskites in paramagnetic state".APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING 104.1(2011):135-142. |
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