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Local chemical ordering within the incubation period as a trigger for nanocrystallization of a highly supercooled Ti-based liquid
Wang, Zhi1,2; Chen, Chunlin1,3; Ketov, Sergey, V1,4; Akagi, Kazuto1; Tsarkov, Andrey A.5; Ikuhara, Yuichi1,6; Louzguine-Luzgin, Dmitri, V1
通讯作者Chen, Chunlin(chen.chunlin@wpi-aimr.tohoku.ac.jp) ; Louzguine-Luzgin, Dmitri, V(dml@wpi-aimr.tohoku.ac.jp)
2018-10-15
发表期刊MATERIALS & DESIGN
ISSN0264-1275
卷号156页码:504-513
摘要In the present work we study nanocrystallization of the Ti50Ni23Cu22Sn5 alloy within the supercooled liquid region by using a state-of-the-art experimental technique with elemental mapping at near-atomic resolution especially focusing on the incubation period which is still poorly understood from both the theoretical and experimental viewpoint. Molecular dynamics (MD) simulation results performed for the Ti55Ni45 liquid acting as a simplified model system of the (Ti,Sn)(55)(Ni,Cu)(45) alloy illustrate the process of nucleation and provide some additional suggestions. The experiment and MD results indicate formation of nanometer-range chemical rearrangements which are supposed to reduce the energy barrier in the complex energy landscape finally leading to a high density of homogeneously nucleating crystallites after the completion of a macroscopically observed incubation period. (C) 2018 Published by Elsevier Ltd.
关键词Nucleation Supercooled liquid Metallic glass Chemical inhomogeneity Energy barrier
资助者World Premier International Research Center Initiative (WPI), MEXT, Japan ; Fusion Research grant Nucleation - structural formation dynamics of nanomaterials from AIMR, Tohoku University, Japan ; Ministry of Education and Science of the Russian Federation ; National Natural Science Foundation of China
DOI10.1016/j.matdes.2018.07.013
收录类别SCI
语种英语
资助项目World Premier International Research Center Initiative (WPI), MEXT, Japan ; Fusion Research grant Nucleation - structural formation dynamics of nanomaterials from AIMR, Tohoku University, Japan ; Ministry of Education and Science of the Russian Federation[K2-2014-013] ; Ministry of Education and Science of the Russian Federation[K2-2017-089] ; National Natural Science Foundation of China[51701075]
WOS研究方向Materials Science
WOS类目Materials Science, Multidisciplinary
WOS记录号WOS:000441422300048
出版者ELSEVIER SCI LTD
引用统计
被引频次:18[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/128787
专题中国科学院金属研究所
通讯作者Chen, Chunlin; Louzguine-Luzgin, Dmitri, V
作者单位1.Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan
2.South China Univ Technol, Sch Mech & Automot Engn, Natl Engn Res Ctr Near Net Shape Forming Metall M, 381 Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China
4.Austrian Acad Sci, Erich Schmid Inst Mat Sci, A-8700 Leoben, Austria
5.Natl Univ Sci & Technol MISiS, Moscow 119049, Russia
6.Univ Tokyo, Inst Engn Innovat, Tokyo 1138656, Japan
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Wang, Zhi,Chen, Chunlin,Ketov, Sergey, V,et al. Local chemical ordering within the incubation period as a trigger for nanocrystallization of a highly supercooled Ti-based liquid[J]. MATERIALS & DESIGN,2018,156:504-513.
APA Wang, Zhi.,Chen, Chunlin.,Ketov, Sergey, V.,Akagi, Kazuto.,Tsarkov, Andrey A..,...&Louzguine-Luzgin, Dmitri, V.(2018).Local chemical ordering within the incubation period as a trigger for nanocrystallization of a highly supercooled Ti-based liquid.MATERIALS & DESIGN,156,504-513.
MLA Wang, Zhi,et al."Local chemical ordering within the incubation period as a trigger for nanocrystallization of a highly supercooled Ti-based liquid".MATERIALS & DESIGN 156(2018):504-513.
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