| The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts | |
| Li, Jin-Cheng1,2; Tang, Dai-Ming1; Hou, Peng-Xiang1; Li, Guo-Xian1; Cheng, Min1; Liu, Chang1; Cheng, Hui-Ming1,3 | |
| Corresponding Author | Hou, Peng-Xiang(pxhou@imr.ac.cn) ; Liu, Chang(cliu@imr.ac.cn) |
| 2018-09-01 | |
| Source Publication | MRS COMMUNICATIONS
 |
| ISSN | 2159-6859 |
| Volume | 8Issue:3Pages:1158-1166 |
| Abstract | Owing to lack of a definitive correlation between carbon supports and catalytic activity of single-atom Fe-active sites, rational design and preparation of single-atom Fe catalysts have so far been elusive. Herein we designed and prepared one-dimensional core-shell nanostructured single-atom Fe catalysts, in which carbon nanofibers and carbon nanotubes with different crystallinities and electrical conductivities were used as supports to host single-atom Fe-active sites. It was found that the carbon supports with higher electrical conductivity accelerate charge transfer and enhance the oxygen reduction reaction (ORR) activity of single-atom Fe-active sites as well as the ORR durability of the final catalyst. |
| Funding Organization | Ministry of Science and Technology of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; CAS/SAFEA International Partnership Program for Creative Research Teams ; Liaoning BaiQianWan Talents Program |
| DOI | 10.1557/mrc.2018.174 |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | Ministry of Science and Technology of China[2016YFA0200102] ; National Natural Science Foundation of China[51625203] ; National Natural Science Foundation of China[51532008] ; National Natural Science Foundation of China[51521091] ; National Natural Science Foundation of China[51772303] ; National Natural Science Foundation of China[51572264] ; Chinese Academy of Sciences[KGZD-EW-T06] ; CAS/SAFEA International Partnership Program for Creative Research Teams ; Liaoning BaiQianWan Talents Program |
| WOS Research Area | Materials Science |
| WOS Subject | Materials Science, Multidisciplinary |
| WOS ID | WOS:000448887900067 |
| Publisher | CAMBRIDGE UNIV PRESS |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imr.ac.cn/handle/321006/130119 |
| Collection | 中国科学院金属研究所 |
| Corresponding Author | Hou, Peng-Xiang; Liu, Chang |
| Affiliation | 1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China 2.Hong Kong Univ Sci & Technol, Fok Ying Tung Res Inst, Guangzhou 511458, Guangdong, Peoples R China 3.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 5108055, Peoples R China |
| Recommended Citation GB/T 7714 | Li, Jin-Cheng,Tang, Dai-Ming,Hou, Peng-Xiang,et al. The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts[J]. MRS COMMUNICATIONS,2018,8(3):1158-1166. |
| APA | Li, Jin-Cheng.,Tang, Dai-Ming.,Hou, Peng-Xiang.,Li, Guo-Xian.,Cheng, Min.,...&Cheng, Hui-Ming.(2018).The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts.MRS COMMUNICATIONS,8(3),1158-1166. |
| MLA | Li, Jin-Cheng,et al."The effect of carbon support on the oxygen reduction activity and durability of single-atom iron catalysts".MRS COMMUNICATIONS 8.3(2018):1158-1166. |
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