UV-Epoxy-Enabled Simultaneous Intact Transfer and Highly Efficient Doping for Roll-to-Roll Production of High-Performance Graphene Films

doi:10.1021/acsami.8b13686

IMR OpenIR

	UV-Epoxy-Enabled Simultaneous Intact Transfer and Highly Efficient Doping for Roll-to-Roll Production of High-Performance Graphene Films
	Ma, Lai-Peng 1; Dong, Shichao 1; Chen, Maolin 1,2; Ma, Wei 1,2; Sun, Dongming 1; Gao, Yang 1; Ma, Teng 1; Cheng, Hui-Ming 1; Ren, Wencai 1
通讯作者	Ren, Wencai(wcren@imr.ac.cn)
	2018-11-28
发表期刊	ACS APPLIED MATERIALS & INTERFACES
ISSN	1944-8244
卷号	10 期号:47 页码:40756-40763
摘要	Flexible graphene transparent conductive films (TCFs) prepared by chemical vapor deposition hold great promise for next-generation wearable optoelectronic devices, but the lack of low-cost scalable intact transfer and highly efficient doping greatly limits their commercialization. Here, we report a UV-epoxy adhesive as a robust multifunctional layer for the low-cost scalable production of high-performance flexible graphene TCF. Its high solvent stability, sufficient adhesion force, and conformal contact with graphene enable the intact bubbling transfer of graphene. More importantly, a highly strong and stable p-dopant, superacid HSbF6, is in situ generated from UV-epoxy. HSbF6 substantially increases the hole concentration of pristine graphene by more than 10 times and consequently reduces its sheet resistance by up to 95% with high stability. Furthermore, it can be readily integrated with the roll-to-roll transfer process. These features enable continuous production of graphene TCFs with overall performances superior to those produced by common transfer methods and typical dopants. As an example, we demonstrate the use of this film in the capacitive multitouch panel of tablet computers.
关键词	flexible transparent electrode graphene adhesive doping roll-to-roll bubbling transfer
资助者	Ministry of Science and Technology of China ; National Science Foundation of China ; Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences
DOI	10.1021/acsami.8b13686
收录类别	SCI
语种	英语
资助项目	Ministry of Science and Technology of China[2016YFA0200101] ; Ministry of Science and Technology of China[2016YFB04001104] ; National Science Foundation of China[51325205] ; National Science Foundation of China[51290273] ; National Science Foundation of China[51521091] ; National Science Foundation of China[51272256] ; National Science Foundation of China[61422406] ; National Science Foundation of China[61574143] ; Chinese Academy of Sciences[KGZD-EW-303-1] ; Chinese Academy of Sciences[KGZD-EW-303-3] ; Chinese Academy of Sciences[KGZD-EW-T06] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB30000000]
WOS研究方向	Science & Technology - Other Topics ; Materials Science
WOS类目	Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000451932800041
出版者	AMER CHEMICAL SOC
引用统计	被引频次：20[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/130589
专题	中国科学院金属研究所
通讯作者	Ren, Wencai
作者单位	1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
推荐引用方式 GB/T 7714	Ma, Lai-Peng,Dong, Shichao,Chen, Maolin,et al. UV-Epoxy-Enabled Simultaneous Intact Transfer and Highly Efficient Doping for Roll-to-Roll Production of High-Performance Graphene Films[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(47):40756-40763.
APA	Ma, Lai-Peng.,Dong, Shichao.,Chen, Maolin.,Ma, Wei.,Sun, Dongming.,...&Ren, Wencai.(2018).UV-Epoxy-Enabled Simultaneous Intact Transfer and Highly Efficient Doping for Roll-to-Roll Production of High-Performance Graphene Films.ACS APPLIED MATERIALS & INTERFACES,10(47),40756-40763.
MLA	Ma, Lai-Peng,et al."UV-Epoxy-Enabled Simultaneous Intact Transfer and Highly Efficient Doping for Roll-to-Roll Production of High-Performance Graphene Films".ACS APPLIED MATERIALS & INTERFACES 10.47(2018):40756-40763.