Defective graphene@diamond hybrid nanocarbon material as an effective and stable metal-free catalyst for acetylene hydrochlorination | |
Lan, Guojun1; Qiu, Yiyang1; Fan, Jiangtao1; Wang, Xiaolong1; Tang, Haodong1; Han, Wenfeng1; Liu, Huazhang1; Liu, Hongyang2; Song, Shuang3; Li, Ying1 | |
通讯作者 | Liu, Hongyang(liuhy@imr.ac.cn) ; Li, Ying(liying@zjut.edu.cn) |
2019-02-04 | |
发表期刊 | CHEMICAL COMMUNICATIONS
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ISSN | 1359-7345 |
卷号 | 55期号:10页码:1430-1433 |
摘要 | A defective nanodiamond-graphene material (ND@G) exhibits superior catalytic activity in acetylene hydrochlorination with an acetylene conversion of 50%, selectivity to vinyl chloride of up to 99.5% at 220 degrees C, and a C2H2 gas hourly space velocity of 300 h(-1), which is the first example of a metal-free catalyst with comparable performance to that of the 0.25% Au/C catalyst. |
资助者 | Natural Science Foundation of China (NSFC) ; Natural Science Foundation of Zhejiang Province ; preferential Foundation of Zhejiang province postdoctoral research project ; Ministry of Science and Technology (MOST) ; National Natural Science Foundation of China ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) |
DOI | 10.1039/c8cc09361j |
收录类别 | SCI |
语种 | 英语 |
资助项目 | Natural Science Foundation of China (NSFC)[21776257] ; Natural Science Foundation of Zhejiang Province[LY17B030010] ; preferential Foundation of Zhejiang province postdoctoral research project ; Ministry of Science and Technology (MOST)[2016YFA0204100] ; National Natural Science Foundation of China[91845201] ; National Natural Science Foundation of China[21573254] ; National Natural Science Foundation of China[91545110] ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Multidisciplinary |
WOS记录号 | WOS:000458546700012 |
出版者 | ROYAL SOC CHEMISTRY |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/132005 |
专题 | 中国科学院金属研究所 |
通讯作者 | Liu, Hongyang; Li, Ying |
作者单位 | 1.Zhejiang Univ Technol, Inst Ind Catalysis, Chaowang Rd 18, Hangzhou, Zhejiang, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Wenhua Rd 72, Shenyang, Liaoning, Peoples R China 3.Zhejiang Univ Technol, Coll Environm, Chaowang Rd 18, Hangzhou, Zhejiang, Peoples R China |
推荐引用方式 GB/T 7714 | Lan, Guojun,Qiu, Yiyang,Fan, Jiangtao,et al. Defective graphene@diamond hybrid nanocarbon material as an effective and stable metal-free catalyst for acetylene hydrochlorination[J]. CHEMICAL COMMUNICATIONS,2019,55(10):1430-1433. |
APA | Lan, Guojun.,Qiu, Yiyang.,Fan, Jiangtao.,Wang, Xiaolong.,Tang, Haodong.,...&Li, Ying.(2019).Defective graphene@diamond hybrid nanocarbon material as an effective and stable metal-free catalyst for acetylene hydrochlorination.CHEMICAL COMMUNICATIONS,55(10),1430-1433. |
MLA | Lan, Guojun,et al."Defective graphene@diamond hybrid nanocarbon material as an effective and stable metal-free catalyst for acetylene hydrochlorination".CHEMICAL COMMUNICATIONS 55.10(2019):1430-1433. |
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