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A hierarchical porous Fe-N impregnated carbon-graphene hybrid for high-performance oxygen reduction reaction
Wang, Sihui1,2; Yan, Xiao1,3; Wu, Kuang-Hsu4; Chen, Xuemin5; Feng, Jian-Min6; Lu, Pengyi7; Feng, Hou7; Cheng, Hui-Ming8; Liang, Ji1; Dou, Shi Xue1
Corresponding AuthorWu, Kuang-Hsu(kuang-hsu.wu@unsw.edu.au) ; Liang, Ji(liangj@uow.edu.au)
2019-04-01
Source PublicationCARBON
ISSN0008-6223
Volume144Pages:798-804
AbstractA Fe-N impregnated carbon in a hybrid with in-situ grown graphene from hierarchical porous carbon has been obtained for high-performance oxygen reduction reaction (ORR) catalysis. This hybrid material combines the desirable characteristics for the ORR, including Fe-N active sites, high surface area, good electron conductivity, and hierarchical channels for mass diffusion. As a result, this catalyst exhibits a very positive reaction onset potential (-0.05 V vs. Ag/AgCl), a high ORR current density, and a complete four-electron ORR pathway, which are even better than a commercial 20% Pt/C catalyst. We further reveal the synergistic ORR enhancement from the controlled Fe-N impregnation in the doped carbon-graphene hybrid. (C) 2018 Elsevier Ltd. All rights reserved.
Funding OrganizationAustralian Research Council under the Discovery Early Career Researcher Award (DECRA) scheme ; China Scholarship Council
DOI10.1016/j.carbon.2018.12.066
Indexed BySCI
Language英语
Funding ProjectAustralian Research Council under the Discovery Early Career Researcher Award (DECRA) scheme[DE170100871] ; China Scholarship Council[201804910018]
WOS Research AreaChemistry ; Materials Science
WOS SubjectChemistry, Physical ; Materials Science, Multidisciplinary
WOS IDWOS:000459991900087
PublisherPERGAMON-ELSEVIER SCIENCE LTD
Citation statistics
Cited Times:37[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/132277
Collection中国科学院金属研究所
Corresponding AuthorWu, Kuang-Hsu; Liang, Ji
Affiliation1.Univ Wollongong, Inst Superconducting & Elect Mat, Australian Inst Innovat Mat, Wollongong, NSW 2500, Australia
2.Tianjin Sino German Univ Appl Sci, Sch Aeronaut & Astronaut, Tianjin 300350, Peoples R China
3.Chinese Acad Sci, Guangdong Key Lab Membrane Mat & Membrane Separat, Guangzhou Inst Adv Technol, Guangzhou 511458, Guangdong, Peoples R China
4.Univ New South Wales, Particles & Catalysis Res Grp, Sch Chem Engn, Sydney, NSW 2052, Australia
5.Hebei Univ Sci & Technol, Sch Sci, Shijiazhuang 050018, Hebei, Peoples R China
6.Tianjin Normal Univ, Energy & Mat Engn Ctr, Coll Phys & Mat Sci, Tianjin 300387, Peoples R China
7.Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China
8.Chinese Acad Sci, Adv Carbon Div, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Wang, Sihui,Yan, Xiao,Wu, Kuang-Hsu,et al. A hierarchical porous Fe-N impregnated carbon-graphene hybrid for high-performance oxygen reduction reaction[J]. CARBON,2019,144:798-804.
APA Wang, Sihui.,Yan, Xiao.,Wu, Kuang-Hsu.,Chen, Xuemin.,Feng, Jian-Min.,...&Dou, Shi Xue.(2019).A hierarchical porous Fe-N impregnated carbon-graphene hybrid for high-performance oxygen reduction reaction.CARBON,144,798-804.
MLA Wang, Sihui,et al."A hierarchical porous Fe-N impregnated carbon-graphene hybrid for high-performance oxygen reduction reaction".CARBON 144(2019):798-804.
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