IMR OpenIR
Electrochemical process of sulfur in carbon materials from electrode thickness to interlayer
Tang, Xiaonan1,2; Sun, Zhenhua2,3; Yang, Huicong2; Fang, Haitao4; Wei, Fei5; Cheng, Hui-Ming2,6; Zhuo, Shuping1; Li, Feng2,3
Corresponding AuthorZhuo, Shuping(zhuosp_academic@yahoo.com) ; Li, Feng(fli@imr.ac.cn)
2019-04-01
Source PublicationJOURNAL OF ENERGY CHEMISTRY
ISSN2095-4956
Volume31Pages:119-124
AbstractLots of efforts have been done on different porous carbon materials as cathode for Lithium-sulfur (Li-S) battery. However, seldom researches have been done on the relationship between cathode thickness and electrochemical performance. Our work investigates the relation between electrochemical performance and cathode thickness with typical porous carbon materials. We explain the phenomenon that only a modest cathode thickness can have the most adequate electrochemical reaction trend through the aspect of thermodynamics (chemical potential) so that the best electrochemical performance can be obtained. Besides, interlayer can remit the shuttle effect but hinder the lithium ion diffusion process simultaneously. And we verify the effect of interlayer thickness on the shuttle effect and lithium ion diffusion process. (C) 2018 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
KeywordLithium-sulfur battery Electrochemical reaction Cathode thickness Chemical potential Ion diffusion
Funding OrganizationNational Key R&D Program of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Institute of Metal Research ; Strategic Priority Research Program of Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; CAS/SAFEA International Partnership Program for Creative Research Teams
DOI10.1016/j.jechem.2018.06.001
Indexed BySCI
Language英语
Funding ProjectNational Key R&D Program of China[2016YFA0200102] ; National Key R&D Program of China[2016YFB0100100] ; National Key R&D Program of China[2014CB932402] ; National Natural Science Foundation of China[51525206] ; National Natural Science Foundation of China[51521091] ; National Natural Science Foundation of China[51372253] ; National Natural Science Foundation of China[U1401243] ; National Natural Science Foundation of China[21576159] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[2015150] ; Institute of Metal Research[2015-PY03] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA09010104] ; Key Research Program of the Chinese Academy of Sciences[KGZD-EW-T06] ; CAS/SAFEA International Partnership Program for Creative Research Teams
WOS Research AreaChemistry ; Energy & Fuels ; Engineering
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS IDWOS:000460174000014
PublisherELSEVIER SCIENCE BV
Citation statistics
Cited Times:24[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/132448
Collection中国科学院金属研究所
Corresponding AuthorZhuo, Shuping; Li, Feng
Affiliation1.Shandong Univ Technol, Sch Chem Engn, Zibo 255049, Shandong, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
4.Harbin Inst Technol, Sch Mat Sci & Engn, Harbin 150001, Heilongjiang, Peoples R China
5.Tsinghua Univ, Dept Chem Engn, Beijing 100084, Peoples R China
6.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Tang, Xiaonan,Sun, Zhenhua,Yang, Huicong,et al. Electrochemical process of sulfur in carbon materials from electrode thickness to interlayer[J]. JOURNAL OF ENERGY CHEMISTRY,2019,31:119-124.
APA Tang, Xiaonan.,Sun, Zhenhua.,Yang, Huicong.,Fang, Haitao.,Wei, Fei.,...&Li, Feng.(2019).Electrochemical process of sulfur in carbon materials from electrode thickness to interlayer.JOURNAL OF ENERGY CHEMISTRY,31,119-124.
MLA Tang, Xiaonan,et al."Electrochemical process of sulfur in carbon materials from electrode thickness to interlayer".JOURNAL OF ENERGY CHEMISTRY 31(2019):119-124.
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