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A Desolvated Solid-Solid-Solid Interface for a High-Capacitance Electric Double Layer
Wang, Yu-Zuo1,2; Shan, Xu-Yi1; Ma, Li-Po3; Wang, Jia-Wei3; Wang, Da-Wei4; Peng, Zhang-Quan3; Cheng, Hui-Ming1,5,6; Li, Feng1,7
Corresponding AuthorWang, Da-Wei(da-wei.wang@unsw.edu.au) ; Li, Feng(fli@imr.ac.cn)
2019-03-27
Source PublicationADVANCED ENERGY MATERIALS
ISSN1614-6832
Volume9Issue:12Pages:6
AbstractUnderstanding the electric double layer is essential for achieving efficient electrochemical energy storage technologies. A conventional solid-liquid electrode interface suffers from serious self-discharge and a narrow voltage window, which makes the development of a solid-solid interface imperative. However, an in-depth understanding of the electric double layer with a solid- solid interface is lacking. Here, a solid-solid interfacial electric double layer is proposed with excellent electrochemical performance. The solid layer is constructed by the electrochemical decomposition of lithium difluora(oxalate) borate, which provides a desolvated environment for the establishment of a electric double layer. This makes a stronger interaction between the electrode surface and the ions. Based on this unique property, it is found that the solid- solid interfacial electric double layer has an increased capacitance, which suggests a way to develop high-energy electrochemical capacitors.
Keywordcapacitance electric double layers solid-solid interfaces
Funding OrganizationNational Science Foundation of China ; Ministry of Science and Technology of China ; Key Research Program of the Chinese Academy of Sciences
DOI10.1002/aenm.201803715
Indexed BySCI
Language英语
Funding ProjectNational Science Foundation of China[51525206] ; National Science Foundation of China[51521091] ; National Science Foundation of China[51372253] ; Ministry of Science and Technology of China[2016YFA0200100] ; Ministry of Science and Technology of China[2016YFB0100100] ; Key Research Program of the Chinese Academy of Sciences[KGZD-EW-T06]
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000463288400011
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Cited Times:6[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/132644
Collection中国科学院金属研究所
Corresponding AuthorWang, Da-Wei; Li, Feng
Affiliation1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China
2.Northeastern Univ, Key Lab Anisotropy & Texture Mat, Shenyang 110819, Liaoning, Peoples R China
3.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China
4.Univ New South Wales, Sch Chem Engn, Sydney, NSW 2052, Australia
5.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China
6.King Abdulaziz Univ, Ctr Excellence Environm Studies, Jeddah 21589, Saudi Arabia
7.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
Recommended Citation
GB/T 7714
Wang, Yu-Zuo,Shan, Xu-Yi,Ma, Li-Po,et al. A Desolvated Solid-Solid-Solid Interface for a High-Capacitance Electric Double Layer[J]. ADVANCED ENERGY MATERIALS,2019,9(12):6.
APA Wang, Yu-Zuo.,Shan, Xu-Yi.,Ma, Li-Po.,Wang, Jia-Wei.,Wang, Da-Wei.,...&Li, Feng.(2019).A Desolvated Solid-Solid-Solid Interface for a High-Capacitance Electric Double Layer.ADVANCED ENERGY MATERIALS,9(12),6.
MLA Wang, Yu-Zuo,et al."A Desolvated Solid-Solid-Solid Interface for a High-Capacitance Electric Double Layer".ADVANCED ENERGY MATERIALS 9.12(2019):6.
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