IMR OpenIR
On-Demand Preparation of alpha-Phase-Dominated Tungsten Films for Highly Qualified Thermal Reflectors
Wang, Xiaoyu1; Zang, Rui1; Gao, Junhua1; Liu, Chen2; Wang, Lei2; Gong, Wenbin3; Zha, Xianhu4; Chen, Xingqiu2; Huang, Feng4; Javaid, Kashif1; Xu, Zhi5; Cao, Hongtao1; Rogachev, Alexander A.6
Corresponding AuthorGao, Junhua(gaojunhua@nimte.ac.cn) ; Cao, Hongtao(h_cao@nimte.ac.cn)
2019-06-01
Source PublicationADVANCED MATERIALS INTERFACES
ISSN2196-7350
Volume6Issue:11Pages:12
AbstractPhase-structure diversity affords tungsten thin films with fascinating physical/chemical properties for varied applications. However, the on-demand preparation of W films with specific phase is still an important but unmet scientific issue. In this report, an easy-to-achieve preparation recipe is implemented for addressing the phase tailoring of tungsten films. The phase transformation evolution during deposition is governed by enhanced diffusion of W adatoms and selective atomic etching on the crystal planes. It is experimentally demonstrated that the orientation relation between {210}(beta) and {110}(alpha) planes plays a vital role in coupling with the competitive growth behaviors between beta- and alpha-W. The phase-dependent electrical/optical properties of W films are experimentally observed and unambiguously figured out by theoretical simulations. Alpha-phase-dominated W films are prepared successfully under relatively tolerant conditions, demonstrating a low resistivity of approximate to 13.6 mu omega cm and a high infrared reflectance larger than 93%. Alpha-W also serves as thermal reflector to construct a solar absorber, exhibiting a low thermal emissivity of approximate to 9.8%@500 degrees C. Understanding the (alpha, beta) phase transformation mechanism means a big step forward in the development of the on-demand preparation, which allows to build a scalable platform for making W films with specific phase in a more controllable way.
Keywordfirst-principles calculation infrared reflectance phase transformation resistivity thermal reflector tungsten thin film
Funding OrganizationNatural Science Foundation of Zhejiang Province ; Key Research and Development Plan of Jiangsu Province ; program for Ningbo Municipal Science and Technology Innovative Research Team ; National Nature Science Foundation of China
DOI10.1002/admi.201900031
Indexed BySCI
Language英语
Funding ProjectNatural Science Foundation of Zhejiang Province[LY17E020012] ; Key Research and Development Plan of Jiangsu Province[BE2015049] ; program for Ningbo Municipal Science and Technology Innovative Research Team[2016B10005] ; National Nature Science Foundation of China[51671193]
WOS Research AreaChemistry ; Materials Science
WOS SubjectChemistry, Multidisciplinary ; Materials Science, Multidisciplinary
WOS IDWOS:000471079000015
PublisherWILEY
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/133917
Collection中国科学院金属研究所
Corresponding AuthorGao, Junhua; Cao, Hongtao
Affiliation1.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Key Lab Graphene Technol & Applicat Zhejiang Prov, Ningbo 315201, Zhejiang, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
3.Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Key Lab Nanodevices & Applicat, Suzhou 215123, Peoples R China
4.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Engn Lab Nucl Energy Mat, Ningbo 315201, Zhejiang, Peoples R China
5.Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China
6.Francisk Skorina Gomel State Univ, Gomel 246019, BELARUS
Recommended Citation
GB/T 7714
Wang, Xiaoyu,Zang, Rui,Gao, Junhua,et al. On-Demand Preparation of alpha-Phase-Dominated Tungsten Films for Highly Qualified Thermal Reflectors[J]. ADVANCED MATERIALS INTERFACES,2019,6(11):12.
APA Wang, Xiaoyu.,Zang, Rui.,Gao, Junhua.,Liu, Chen.,Wang, Lei.,...&Rogachev, Alexander A..(2019).On-Demand Preparation of alpha-Phase-Dominated Tungsten Films for Highly Qualified Thermal Reflectors.ADVANCED MATERIALS INTERFACES,6(11),12.
MLA Wang, Xiaoyu,et al."On-Demand Preparation of alpha-Phase-Dominated Tungsten Films for Highly Qualified Thermal Reflectors".ADVANCED MATERIALS INTERFACES 6.11(2019):12.
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