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Overview of the synthesis of MXenes and other ultrathin 2D transition metal carbides and nitrides
Verger, Louisiane1; Xu, Chuan2; Natu, Varun1; Cheng, Hui-Ming2,3; Ren, Wencai2,3; Barsoum, Michel W.1
通讯作者Ren, Wencai(wcren@imr.ac.cn) ; Barsoum, Michel W.(barsoumw@drexel.edu)
2019-06-01
发表期刊CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE
ISSN1359-0286
卷号23期号:3页码:149-163
摘要In 2011, a new family of two dimensional (2D) carbides, carbonitrides and nitrides - labeled MXenes - was discovered. Since then the number of papers on these materials has increased exponentially for several reasons amongst them: their hydrophilic nature, excellent electronic conductivities and ease of synthesizing large quantities in water. This unique combination of properties and ease of processing has positioned them as enabling materials for a large, and quite varied, host of applications from energy storage to electromagnetic shielding, transparent conductive electrodes, electrocatalysis, to name a few. Since the initial synthesis of Ti3C2 in hydrofluoric acid, many more compositions were discovered, and different synthesis pathways were explored. Most of the work done so far has been conducted on top-down synthesis where a layered parent compound is etched and then exfoliated. Three bottom-up synthesis methods, chemical vapor deposition, a template method and plasma enhanced pulsed laser deposition have been reported. The latter methods enable the synthesis of not only high-quality ultrathin 2D transition metal carbide and nitride films, but also those that could not be synthesized by selective etching. This article reviews and summarizes the most important breakthroughs in the synthesis of MXenes and high-quality ultrathin 2D transition metal carbide and nitride films.
关键词MXenes 2D materials Top-down synthesis Bottom-up synthesis
资助者Swedish Research Council ; National Science Foundation of China ; Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; SYNL-T.S. K Research Fellowship ; Youth Innovation Promotion Association of Chinese Academy of Sciences
DOI10.1016/j.cossms.2019.02.001
收录类别SCI
语种英语
资助项目Swedish Research Council[621-2014-4890] ; National Science Foundation of China[51325205] ; National Science Foundation of China[51290273] ; National Science Foundation of China[51521091] ; Chinese Academy of Sciences[KGZD-EW-T06] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB30000000] ; SYNL-T.S. K Research Fellowship ; Youth Innovation Promotion Association of Chinese Academy of Sciences
WOS研究方向Materials Science ; Physics
WOS类目Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:000483415300004
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:337[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/135189
专题中国科学院金属研究所
通讯作者Ren, Wencai; Barsoum, Michel W.
作者单位1.Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Peoples R China
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Verger, Louisiane,Xu, Chuan,Natu, Varun,et al. Overview of the synthesis of MXenes and other ultrathin 2D transition metal carbides and nitrides[J]. CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE,2019,23(3):149-163.
APA Verger, Louisiane,Xu, Chuan,Natu, Varun,Cheng, Hui-Ming,Ren, Wencai,&Barsoum, Michel W..(2019).Overview of the synthesis of MXenes and other ultrathin 2D transition metal carbides and nitrides.CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE,23(3),149-163.
MLA Verger, Louisiane,et al."Overview of the synthesis of MXenes and other ultrathin 2D transition metal carbides and nitrides".CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE 23.3(2019):149-163.
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