Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting

doi:10.1021/acsami.9b21793

IMR OpenIR

	Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting
	Li, Jing 1; Yang, Wenjin 1; Wu, Aimin 2; Zhang, Xinglai 1; Xu, Tingting 1; Liu, Baodan 1
通讯作者	Liu, Baodan(baodanliu@hotmail.com)
	2020-02-19
发表期刊	ACS APPLIED MATERIALS & INTERFACES
ISSN	1944-8244
卷号	12 期号:7 页码:8583-8591
摘要	y A (GaN)(1-x)(ZnO)(x) solid solution as a promising visible-light-driven photocatalyst for overall water splitting has attracted extensive attention. In this work, we proposed a template reactive strategy toward the synthesis of band-gap tunable 2D (GaN)(1-x)(ZnO)(x) nanosheets as thin as 14 nm to reduce the carrier transportation path and thus efficiently decrease the recombination of electrons and holes. It is demonstrated that the template strategy enables an ideal morphology and structure transformation from hexagonal 2D ZnGa2O4 nanosheets to 2D (GaN)(1-x)(ZnO)(x) nanosheets in the nitridation process. After the modification of 1 wt % of Rh cocatalyst, the flowerlike (GaN)(0.89)(ZnO)(0.11) nanosheets show an enhanced hydrogen evolution in pure water (pH 4.5).
关键词	(GaN)(1-x)(ZnO)(x) solid solution nanosheets photocatalytic water splitting
资助者	National Natural Science Foundation of China
DOI	10.1021/acsami.9b21793
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51702326] ; National Natural Science Foundation of China[51872296]
WOS研究方向	Science & Technology - Other Topics ; Materials Science
WOS类目	Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000515214300079
出版者	AMER CHEMICAL SOC
引用统计	被引频次：36[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/137331
专题	中国科学院金属研究所
通讯作者	Liu, Baodan
作者单位	1.Chinese Acad Sci, IMR, Shenyang Natl Lab Mat Sci SYNL, Shenyang 110016, Peoples R China 2.Dalian Univ Technol, Key Lab Mat Modificat Laser Ion & Elect Beams, Minist Educ, Dalian 116024, Peoples R China
推荐引用方式 GB/T 7714	Li, Jing,Yang, Wenjin,Wu, Aimin,et al. Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting[J]. ACS APPLIED MATERIALS & INTERFACES,2020,12(7):8583-8591.
APA	Li, Jing,Yang, Wenjin,Wu, Aimin,Zhang, Xinglai,Xu, Tingting,&Liu, Baodan.(2020).Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting.ACS APPLIED MATERIALS & INTERFACES,12(7),8583-8591.
MLA	Li, Jing,et al."Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting".ACS APPLIED MATERIALS & INTERFACES 12.7(2020):8583-8591.