| Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol | |
| Zhao, Zhiliang1; Zhang, Jing1; Wang, Yongzhao2; Guo, Wenyao1; Lv, Lin1; Li, Baiyu3; Zheng, Kang1; Bo, Tingting1; Peng, Dengchao1; Zhou, Zhiyuan1; Zhang, Bingsen2; Shao, Lidong1 | |
| Corresponding Author | Guo, Wenyao(guowenyao@shiep.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn) |
| 2020-05-01 | |
| Source Publication | CHEMICAL PHYSICS LETTERS
 |
| ISSN | 0009-2614 |
| Volume | 746Pages:6 |
| Abstract | In this work, Pd/reduced graphene oxide (Pd/RGO) aerogels, with large surface areas and wrinkles, are obtained through the lyophilisation, vacuum and reduction treatments. Pd/RGO aerogels exhibit higher catalytic performances and thermal stability in comparison to the reference catalyst Pd/activated carbon (Pd/AC) in the oxidation of benzyl alcohol. The surface analyses indicate that Pd/RGO aerogels possess a higher proportion of Pd2+ than the Pd/AC catalyst. Meanwhile, the oxygen-containing functional groups can modulate the interaction between palladium and the support to form active phases for the reaction. Moreover, Pd nanoparticles (PdNPs) remain well dispersed in nanoscale on the reacted Pd/RGO aerogels. |
| Keyword | Pd nanoparticles Solvent-free oxidation Benzyl alcohol Graphene oxide Aerogel |
| Funding Organization | National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program |
| DOI | 10.1016/j.cplett.2020.137306 |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | National Natural Science Foundation of China[21773269] ; Liao Ning Revitalization Talents Program[XLYC1807175] |
| WOS Research Area | Chemistry ; Physics |
| WOS Subject | Chemistry, Physical ; Physics, Atomic, Molecular & Chemical |
| WOS ID | WOS:000522555600027 |
| Publisher | ELSEVIER |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imr.ac.cn/handle/321006/137851 |
| Collection | 中国科学院金属研究所 |
| Corresponding Author | Guo, Wenyao; Zhang, Bingsen; Shao, Lidong |
| Affiliation | 1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China 2.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China 3.Nantong Vocat Univ, 89 Qingnian Rd, Nantong 226006, Peoples R China |
| Recommended Citation GB/T 7714 | Zhao, Zhiliang,Zhang, Jing,Wang, Yongzhao,et al. Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol[J]. CHEMICAL PHYSICS LETTERS,2020,746:6. |
| APA | Zhao, Zhiliang.,Zhang, Jing.,Wang, Yongzhao.,Guo, Wenyao.,Lv, Lin.,...&Shao, Lidong.(2020).Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol.CHEMICAL PHYSICS LETTERS,746,6. |
| MLA | Zhao, Zhiliang,et al."Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol".CHEMICAL PHYSICS LETTERS 746(2020):6. |
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