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Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol
Zhao, Zhiliang1; Zhang, Jing1; Wang, Yongzhao2; Guo, Wenyao1; Lv, Lin1; Li, Baiyu3; Zheng, Kang1; Bo, Tingting1; Peng, Dengchao1; Zhou, Zhiyuan1; Zhang, Bingsen2; Shao, Lidong1
Corresponding AuthorGuo, Wenyao(guowenyao@shiep.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
2020-05-01
Source PublicationCHEMICAL PHYSICS LETTERS
ISSN0009-2614
Volume746Pages:6
AbstractIn this work, Pd/reduced graphene oxide (Pd/RGO) aerogels, with large surface areas and wrinkles, are obtained through the lyophilisation, vacuum and reduction treatments. Pd/RGO aerogels exhibit higher catalytic performances and thermal stability in comparison to the reference catalyst Pd/activated carbon (Pd/AC) in the oxidation of benzyl alcohol. The surface analyses indicate that Pd/RGO aerogels possess a higher proportion of Pd2+ than the Pd/AC catalyst. Meanwhile, the oxygen-containing functional groups can modulate the interaction between palladium and the support to form active phases for the reaction. Moreover, Pd nanoparticles (PdNPs) remain well dispersed in nanoscale on the reacted Pd/RGO aerogels.
KeywordPd nanoparticles Solvent-free oxidation Benzyl alcohol Graphene oxide Aerogel
Funding OrganizationNational Natural Science Foundation of China ; Liao Ning Revitalization Talents Program
DOI10.1016/j.cplett.2020.137306
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[21773269] ; Liao Ning Revitalization Talents Program[XLYC1807175]
WOS Research AreaChemistry ; Physics
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000522555600027
PublisherELSEVIER
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/137851
Collection中国科学院金属研究所
Corresponding AuthorGuo, Wenyao; Zhang, Bingsen; Shao, Lidong
Affiliation1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China
2.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China
3.Nantong Vocat Univ, 89 Qingnian Rd, Nantong 226006, Peoples R China
Recommended Citation
GB/T 7714
Zhao, Zhiliang,Zhang, Jing,Wang, Yongzhao,et al. Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol[J]. CHEMICAL PHYSICS LETTERS,2020,746:6.
APA Zhao, Zhiliang.,Zhang, Jing.,Wang, Yongzhao.,Guo, Wenyao.,Lv, Lin.,...&Shao, Lidong.(2020).Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol.CHEMICAL PHYSICS LETTERS,746,6.
MLA Zhao, Zhiliang,et al."Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol".CHEMICAL PHYSICS LETTERS 746(2020):6.
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