Phase-separated Ce-Co-O catalysts for CO oxidation
Zhang, Ruishi1; Wang, Junchao2,3; Zhu, Xiuhui1; Liu, Xiaoyuan2; Liu, Haiyan1; Zhou, Yang2; Dong, Shizhi3; La, Peiqing4; Yao, Jinlei5; Liu, Baodan2
Corresponding AuthorZhu, Xiuhui( ; Liu, Baodan(
AbstractAs a major gas pollutant, the control of CO gas emission from chemical industry and vehicle exhausts has aroused global attention in the past years and it is extremely essential to develop efficient, low-cost and environmental friendly catalysts for CO conversion and removal. In this work, we report the facile synthesis of Ce-Co-O catalysts through a simple ultrasonic spray pyrolysis process and investigate their application for low-temperature CO oxidation. The Ce-Co-O catalysts comprising of separated CeO2 and Co3O4 phases show superior CO oxidation capability below 473 K (200 degrees C) without the assistance of any other co-catalyst or noble metal. With the increase of Co3O4 concentration, the CO oxidation temperature of Ce-Co-O catalysts decreases quickly and reaches a complete conversion temperature of 410 K (137 degrees C) in the case of the optimized Co content. Microstructure analysis using high-resolution transmission electron microscope reveals that the tiny CeO2 and Co3O4 phases assembled into porous particles are well crystallized and show high chemical purity. The porous feature of Ce-Co-O catalysts synthesized from feasible ultrasonic spray pyrolysis makes them more competitive and promising towards gaseous environmental pollution processing including CO oxidation, TWCs, SCR, etc. (C) 2020 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
KeywordCe-Co-O catalysts Phase separation Porous structure Pyrolysis synthesis CO oxidation
Funding OrganizationNational Natural Science Foundation of China ; Shenyang National Laboratory for Materials Science ; State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals
Indexed BySCI
Funding ProjectNational Natural Science Foundation of China[51872296] ; Shenyang National Laboratory for Materials Science[18LHPY012] ; State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals[18LHPY012]
WOS Research AreaChemistry ; Electrochemistry ; Energy & Fuels
WOS SubjectChemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS IDWOS:000526115700013
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Cited Times:9[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Corresponding AuthorZhu, Xiuhui; Liu, Baodan
Affiliation1.Yingkou Inst Technol, Dept Chem & Mat Engn, 46 Bowen Rd, Yingkou 115014, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci SYNL, 72 Wenhua Rd, Shenyang 110016, Peoples R China
3.Liaoning Tech Univ, Sch Mat Sci & Engn, 47 Zhonghua Rd, Fuxing 123000, Peoples R China
4.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China
5.Suzhou Univ Sci & Technol, Sch Math & Phys, Jiangsu Key Lab Micro & Nano Heat Fluid Flow Tech, Suzhou 215009, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Ruishi,Wang, Junchao,Zhu, Xiuhui,et al. Phase-separated Ce-Co-O catalysts for CO oxidation[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2020,45(23):12777-12786.
APA Zhang, Ruishi.,Wang, Junchao.,Zhu, Xiuhui.,Liu, Xiaoyuan.,Liu, Haiyan.,...&Liu, Baodan.(2020).Phase-separated Ce-Co-O catalysts for CO oxidation.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,45(23),12777-12786.
MLA Zhang, Ruishi,et al."Phase-separated Ce-Co-O catalysts for CO oxidation".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 45.23(2020):12777-12786.
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