Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation

doi:10.1016/j.jmst.2019.12.012

IMR OpenIR

	Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation
	Zhao, Bowen 1,2; Zhu, Zhengwang 1; Qin, Xin Dong 3; Li, Zhengkun 1; Zhang, Haifeng 1
通讯作者	Zhu, Zhengwang(zwzhu@imr.ac.cn)
	2020-06-01
发表期刊	JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
ISSN	1005-0302
卷号	46 页码:88-97
摘要	Metallic glasses with the unique disordered atomic structure and metastable nature have been recently applied to degrade the azo dyes and other organic pollutants based on their superior catalytic performance. In this work, the functional properties of six CuZr-based metallic glassy ribbons with the different nominal components in degrading Acid Orange II (AO II) azo dyes were investigated. The Cu47.5Zr46Al6.5 metallic glassy ribbons could exhibit the more advanced catalytic performance for degradation process, which could completely degrade azo dye aqueous solution within 30 min. Additionally, the Cu47.5Zr46Al6.5 metallic glassy ribbons also showed the excellent cyclic stability along with approximately 97.68% degradation efficiency after 10 cycles. These excellent catalytic performance and stability are closely related to the synergistic effect of exposed copper nanoparticles and produced copper oxides in the reaction, which contributes to accelerate the generation of more hydroxyl radicals (OH) to react with dye molecules. Our findings can be able to develop a novel potential metallic glassy material for the functional application of wastewater treatment. (C) 2020 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
关键词	Metallic glasses Catalytic performance Degradation Azo dyes
资助者	National Natural Science Foundation of China ; LiaoNing Revitalization Talents Program ; Shenyang National Laboratory for Materials Science ; Dong Guan Innovative Research Team Program ; Shenyang Amorphous Metal Manufacturing Co., Ltd., Shenyang, China
DOI	10.1016/j.jmst.2019.12.012
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51801209] ; National Natural Science Foundation of China[51790484] ; National Natural Science Foundation of China[U1738101] ; LiaoNing Revitalization Talents Program[XLYC1802078] ; LiaoNing Revitalization Talents Program[XLYC1807062] ; Shenyang National Laboratory for Materials Science ; Dong Guan Innovative Research Team Program[2014607134] ; Shenyang Amorphous Metal Manufacturing Co., Ltd., Shenyang, China
WOS研究方向	Materials Science ; Metallurgy & Metallurgical Engineering
WOS类目	Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS记录号	WOS:000525326000009
出版者	JOURNAL MATER SCI TECHNOL
引用统计	被引频次：30[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/138310
专题	中国科学院金属研究所
通讯作者	Zhu, Zhengwang
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 3.Liaoning Univ, Coll Chem, Inst Rare & Scattered Elements, Shenyang 110036, Peoples R China
推荐引用方式 GB/T 7714	Zhao, Bowen,Zhu, Zhengwang,Qin, Xin Dong,et al. Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2020,46:88-97.
APA	Zhao, Bowen,Zhu, Zhengwang,Qin, Xin Dong,Li, Zhengkun,&Zhang, Haifeng.(2020).Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,46,88-97.
MLA	Zhao, Bowen,et al."Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 46(2020):88-97.