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Polar meron lattice in strained oxide ferroelectrics
Wang, Y. J.1; Feng, Y. P.1,2; Zhu, Y. L.1; Tang, Y. L.1; Yang, L. X.1; Zou, M. J.1,3; Geng, W. R.1,3; Han, M. J.1,2; Guo, X. W.1,3; Wu, B.1; Ma, X. L.1,4
Corresponding AuthorZhu, Y. L.(ylzhu@imr.ac.cn) ; Ma, X. L.(xlma@imr.ac.cn)
2020-06-01
Source PublicationNATURE MATERIALS
ISSN1476-1122
Volume19Issue:8Pages:18
AbstractMerons are topological structures, but these have yet to be directly observed in ferroelectrics. Here, by epitaxially straining PbTiO3 on a SmScO3 substrate, electron microscopy and phase-field modelling allow the morphology and distribution of merons to be observed. A topological meron features a non-coplanar structure, whose order parameters in the core region are perpendicular to those near the perimeter. A meron is half of a skyrmion, and both have potential applications for information carrying and storage. Although merons and skyrmions in ferromagnetic materials can be readily obtained via inter-spin interactions, their behaviour and even existence in ferroelectric materials are still elusive. Here we observe using electron microscopy not only the atomic morphology of merons with a topological charge of 1/2, but also a periodic meron lattice in ultrathin PbTiO3 films under tensile epitaxial strain on a SmScO3 substrate. Phase-field simulations rationalize the formation of merons for which an epitaxial strain, as a single alterable parameter, plays a critical role in the coupling of lattice and charge. This study suggests that by engineering strain at the nanoscale it should be possible to fabricate topological polar textures, which in turn could facilitate the development of nanoscale ferroelectric devices.
Funding OrganizationKey Research Program of Frontier Sciences CAS ; National Natural Science Foundation of China ; Shenyang National Laboratory for Materials Science ; Youth Innovation Promotion Association CAS
DOI10.1038/s41563-020-0694-8
Indexed BySCI
Language英语
Funding ProjectKey Research Program of Frontier Sciences CAS[QYZDJ-SSW-JSC010] ; National Natural Science Foundation of China[51671194] ; National Natural Science Foundation of China[51971223] ; National Natural Science Foundation of China[51922100] ; Shenyang National Laboratory for Materials Science[L2019R06] ; Shenyang National Laboratory for Materials Science[L2019R08] ; Shenyang National Laboratory for Materials Science[L2019F01] ; Shenyang National Laboratory for Materials Science[L2019F13] ; Youth Innovation Promotion Association CAS[2016177]
WOS Research AreaChemistry ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000537030200001
PublisherNATURE PUBLISHING GROUP
Citation statistics
Cited Times:150[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/139167
Collection中国科学院金属研究所
Corresponding AuthorZhu, Y. L.; Ma, X. L.
Affiliation1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang, Peoples R China
2.Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei, Peoples R China
4.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou, Peoples R China
Recommended Citation
GB/T 7714
Wang, Y. J.,Feng, Y. P.,Zhu, Y. L.,et al. Polar meron lattice in strained oxide ferroelectrics[J]. NATURE MATERIALS,2020,19(8):18.
APA Wang, Y. J..,Feng, Y. P..,Zhu, Y. L..,Tang, Y. L..,Yang, L. X..,...&Ma, X. L..(2020).Polar meron lattice in strained oxide ferroelectrics.NATURE MATERIALS,19(8),18.
MLA Wang, Y. J.,et al."Polar meron lattice in strained oxide ferroelectrics".NATURE MATERIALS 19.8(2020):18.
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