Cellulose nanocrystals (CNCs) as hard templates for preparing mesoporous zeolite Y assemblies with high catalytic activity | |
Abdulridha, Samer1; Jiang, Jiuxing2; Xu, Shaojun1; Zhou, Zhaoxia3; Liang, He4; Mao, Boyang5; Zhou, Yangtao6; Garforth, Arthur A.1; Jiao, Yilai1,6; Fan, Xiaolei1 | |
通讯作者 | Jiao, Yilai(yljiao@imr.ac.cn) ; Fan, Xiaolei(xiaolei.fan@manchester.ac.uk) |
2020-08-07 | |
发表期刊 | GREEN CHEMISTRY
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ISSN | 1463-9262 |
卷号 | 22期号:15页码:5115-5122 |
摘要 | Faujasite (FAU) Y zeolite assemblies with high mesoporosity (S-ext= 347 m(2)g(-1)andV(meso)= 0.52 cm(3)g(-1)) were synthesised using sustainable and economic cellulose nanocrystals (CNCs)viaa template-directed synthesis method,i.e.CNCs-Y. In comparison with the control zeolite catalysts of the conventional microporous Y and carbon nanotube templated Y (CNTs-Y) zeolites, the resulting CNCs-Y demonstrated superior performance in catalytic dealkylation with excellent activity and longevity, as well as the anti-coking ability thanks to the exceptional mesoporous features of CNCs-Y zeolites. Thereby, the method and relevant CNCs-Y mesoporous zeolites based on the sustainable CNCs presented here have significant implications for being developed further for improving the sustainability of relevant catalytic processes such as fluid catalytic cracking (FCC). |
资助者 | European Union ; Higher Committee for Education Development in Iraq ; Liaoning Provincial Natural Science Foundation of China ; China Scholarship Council (CSC) |
DOI | 10.1039/d0gc01070g |
收录类别 | SCI |
语种 | 英语 |
资助项目 | European Union[872102] ; Higher Committee for Education Development in Iraq ; Liaoning Provincial Natural Science Foundation of China[20180510012] ; China Scholarship Council (CSC)[201604910181] |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics |
WOS类目 | Chemistry, Multidisciplinary ; Green & Sustainable Science & Technology |
WOS记录号 | WOS:000555342200027 |
出版者 | ROYAL SOC CHEMISTRY |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/140095 |
专题 | 中国科学院金属研究所 |
通讯作者 | Jiao, Yilai; Fan, Xiaolei |
作者单位 | 1.Univ Manchester, Dept Chem Engn & Analyt Sci, Sch Engn, Manchester M13 9PL, Lancs, England 2.Sun Yat Sen Univ, Sch Chem, MOE Key Lab Bioinorgan & Synthet Chem Environm, Guangzhou 510275, Peoples R China 3.Loughborough Univ, Loughborough Mat Characterisat Ctr, Loughborough LE11 3TU, Leics, England 4.Univ Liverpool, Inst Lift Course & Med Sci, Dept Eye & Vis Sci, 6 West Derby St, Liverpool L7 8TX, Merseyside, England 5.Univ Cambridge, Dept Engn, JJ Thomson Ave, Cambridge CB3 0FA, England 6.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China |
推荐引用方式 GB/T 7714 | Abdulridha, Samer,Jiang, Jiuxing,Xu, Shaojun,et al. Cellulose nanocrystals (CNCs) as hard templates for preparing mesoporous zeolite Y assemblies with high catalytic activity[J]. GREEN CHEMISTRY,2020,22(15):5115-5122. |
APA | Abdulridha, Samer.,Jiang, Jiuxing.,Xu, Shaojun.,Zhou, Zhaoxia.,Liang, He.,...&Fan, Xiaolei.(2020).Cellulose nanocrystals (CNCs) as hard templates for preparing mesoporous zeolite Y assemblies with high catalytic activity.GREEN CHEMISTRY,22(15),5115-5122. |
MLA | Abdulridha, Samer,et al."Cellulose nanocrystals (CNCs) as hard templates for preparing mesoporous zeolite Y assemblies with high catalytic activity".GREEN CHEMISTRY 22.15(2020):5115-5122. |
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