Photocatalytic degradation of phenanthrene on soil surfaces in the presence of nanometer anatase TiO2 under UV-light | |
其他题名 | Photocatalytic degradation of phenanthrene on soil surfaces in the presence of nanometer anatase TiO2 under UV-light |
Gu Jiali1; Dong Dianbo2; Kong Lingxue3; Zheng Yong4; Li Xiaojun5 | |
2012 | |
发表期刊 | JOURNAL OF ENVIRONMENTAL SCIENCES
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ISSN | 1001-0742 |
卷号 | 24期号:12页码:2122-2126 |
摘要 | The effect of nanometer anatase TiO2 was investigated on the photocatalytic degradation of phenanthrene on soil surfaces under a variety of conditions. After being spiked with phenanthrene, soil samples loaded with different amounts of TiO2 (0 wt.%, 1 wt.%, 2 wt.%, 3 wt.%, and 4 wt.%) were exposed to UV-light irradiation for 25 hr. The results indicated that the photocatalytic degradation of phenanthrene followed the pseudo first-order kinetics. TiO2 significantly accelerated the degradation of phenanthrene with the half-life reduced from 45.90 to 31.36 hr for TiO2 loading of 0 wt.% and 4 wt.%, respectively. In addition, the effects of H2O2, light intensity and humic acid on the degradation of phenanthrene were investigated. The degradation of phenanthrene increased with the concentration of H2O2, light intensity and the concentration of humic acids. It has been demonstrated that the photocatalytic method in the presence of nanometer anatase TiO2 was a very promising technology for the treatments of soil polluted with organic substances in the future. |
其他摘要 | The effect of nanometer anatase TiO_2 was investigated on the photocatalytic degradation of phenanthrene on soil surfaces under a variety of conditions.After being spiked with phenanthrene,soil samples loaded with different amounts of TiO_2(0wt.%,1wt.%,2wt.%,3wt.%,and 4 wt.%) were exposed to UV-light irradiation for 25 hr.The results indicated that the photocatalytic degradation of phenanthrene followed the pseudo first-order kinetics.TiO_2 significantly accelerated the degradation of phenanthrene with the half-life reduced from 45.90 to 31.36hr for TiO_2 loading of 0wt.% and 4wt.%,respectively.In addition,the effects of H_2O_2,light intensity and humic acid on the degradation of phenanthrene were investigated.The degradation of phenanthrene increased with the concentration of H_2O_2,light intensity and the concentration of humic acids.It has been demonstrated that the photocatalytic method in the presence of nanometer anatase TiO_2 was a very promising technology for the treatments of soil polluted with organic substances in the future. |
关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS HUMIC SUBSTANCES TIO2/WATER INTERFACES CONTAMINATED SOIL SOLID-PHASE PHOTODEGRADATION PHOTOLYSIS PYRENE POLLUTION ATRAZINE nanometer anatase TiO2 photocatalytic degradation phenanthrene soil surfaces UV-light |
收录类别 | CSCD |
语种 | 英语 |
资助项目 | [Open Foundation of Key Laboratory of Industrial Ecology and Environmental Engineering] ; [Liaoning Doctoral Funds] |
CSCD记录号 | CSCD:4710403 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/147645 |
专题 | 中国科学院金属研究所 |
作者单位 | 1.渤海大学 2.中国科学院金属研究所 3.Deakin Univ, Institute Frontier Mat, Geelong, Vic 3217, Australia 4.辽宁大学 5.中国科学院 |
推荐引用方式 GB/T 7714 | Gu Jiali,Dong Dianbo,Kong Lingxue,et al. Photocatalytic degradation of phenanthrene on soil surfaces in the presence of nanometer anatase TiO2 under UV-light[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2012,24(12):2122-2126. |
APA | Gu Jiali,Dong Dianbo,Kong Lingxue,Zheng Yong,&Li Xiaojun.(2012).Photocatalytic degradation of phenanthrene on soil surfaces in the presence of nanometer anatase TiO2 under UV-light.JOURNAL OF ENVIRONMENTAL SCIENCES,24(12),2122-2126. |
MLA | Gu Jiali,et al."Photocatalytic degradation of phenanthrene on soil surfaces in the presence of nanometer anatase TiO2 under UV-light".JOURNAL OF ENVIRONMENTAL SCIENCES 24.12(2012):2122-2126. |
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