Synthesis of high quality nitrogen-doped single-wall carbon nanotubes | |
其他题名 | Synthesis of high quality nitrogen-doped single-wall carbon nanotubes |
Hou Pengxiang; Song Man; Li Jincheng; Liu Chang; Li Shisheng; Cheng Huiming | |
2015 | |
发表期刊 | Science China. Materials
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ISSN | 2095-8226 |
卷号 | 58期号:8页码:603-610 |
摘要 | Nitrogen-doped single-wall carbon nanotubes (SWCNTs) with diameters in the range of 1.1–1.6 nm were synthesized on a large scale by floating catalyst chemical vapor deposition. Ferrocene, methane and melamine were respectively used as the catalyst precursor, carbon source and nitrogen source. The content of nitrogen introduced into the SWCNT lattice was characterized to be ~0.4 at.%. This resulted in a decreased mean diameter, narrower tube diameter distribution, and increased surface area of the SWCNTs. The temperatures at which the rate of weight loss reaches the maximum value for N-SWCNTs are ~785°C, similar to that of pure SWCNTs, indicative of their high-quality and good crystallinity. These N-SWCNTs exhibited a metallic behavior and desirable electrochemical oxygen reduction reaction activity. |
其他摘要 | Nitrogen-doped single-wall carbon nanotubes (SWCNTs) with diameters in the range of 1.1–1.6 nm were synthesized on a large scale by floating catalyst chemical vapor deposition. Ferrocene, methane and melamine were respectively used as the catalyst precursor, carbon source and nitrogen source. The content of nitrogen introduced into the SWCNT lattice was characterized to be ~0.4 at.%. This resulted in a decreased mean diameter, narrower tube diameter distribution, and increased surface area of the SWCNTs. The temperatures at which the rate of weight loss reaches the maximum value for N-SWCNTs are ~785°C, similar to that of pure SWCNTs, indicative of their high-quality and good crystallinity. These N-SWCNTs exhibited a metallic behavior and desirable electrochemical oxygen reduction reaction activity. |
收录类别 | CSCD |
语种 | 英语 |
CSCD记录号 | CSCD:5530248 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/158085 |
专题 | 中国科学院金属研究所 |
作者单位 | 中国科学院金属研究所 |
推荐引用方式 GB/T 7714 | Hou Pengxiang,Song Man,Li Jincheng,et al. Synthesis of high quality nitrogen-doped single-wall carbon nanotubes[J]. Science China. Materials,2015,58(8):603-610. |
APA | Hou Pengxiang,Song Man,Li Jincheng,Liu Chang,Li Shisheng,&Cheng Huiming.(2015).Synthesis of high quality nitrogen-doped single-wall carbon nanotubes.Science China. Materials,58(8),603-610. |
MLA | Hou Pengxiang,et al."Synthesis of high quality nitrogen-doped single-wall carbon nanotubes".Science China. Materials 58.8(2015):603-610. |
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