| Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites | |
| Zou Run1; Dong Xiao1; Jiao Yilai2; D'Agostino, Carmine1; Yan Wenfu3; Fan Xiaolei1 | |
| Corresponding Author | Fan Xiaolei(xiaolei.fan@manchester.ac.uk) |
| 2021-01-10 | |
| Source Publication | CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
 |
| ISSN | 0251-0790 |
| Volume | 42Issue:1Pages:74-100 |
| Abstract | Hierarchical zeolites refer to zeolitic materials having bi-/multi-modal interconnective pores arranged in order of certain ranks, which improve the molecular diffusion within their frameworks, and hence the performance in their applications such as adsorption and heterogeneous catalysis. Hierarchical zeolites are commonly produced via the top-down post-synthetic treatments (such as dealumination and/or desilication) of pre-synthesized zeolites (i.e. the parent zeolites) and the bottom-up synthesis-by-design methods (such as soft/ hard templating). This review presents the recent advances (mainly post 2000) in the strategies of making hierarchical zeolites, with the emphasis on the top-down approaches due to their relatively high practicality. Since hierarchical zeolites are proposed to improve intracrystalline diffusion, experimental studies of guest molecules diffusion in hierarchical zeolites are also reviewed. Additionally, catalytic applications of hierarchical zeolites, in comparison with the conventional microporous pristine zeolites, are also commented to highlight the advantages of hierarchical zeolites to improve catalysis. |
| Keyword | Hierarchical zeolite Post-synthetic treatment Diffusion Pulsed-field gradient nuclear magnetic resonance( PFG NMR) Catalysis |
| Funding Organization | European Union ; China Scholarship Council-The University of Manchester Joint Scholarship ; Programme of Introducing Talents of Discipline to Universities of China ; National Natural Science Foundation of China ; EPSRC New Investigator Award ; Natural Science Foundation of Liaoning Province,China ; National Key Research and Development Program of China |
| DOI | 10.7503/cjcu20200461 |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | European Union[872102] ; China Scholarship Council-The University of Manchester Joint Scholarship[201906740020] ; Programme of Introducing Talents of Discipline to Universities of China[B17020] ; National Natural Science Foundation of China[U1967215] ; National Natural Science Foundation of China[21835002] ; National Natural Science Foundation of China[21621001] ; EPSRC New Investigator Award[EP/S019138/1] ; Natural Science Foundation of Liaoning Province,China[2018010047-301] ; National Key Research and Development Program of China[SQ2019YFE011366] |
| WOS Research Area | Chemistry |
| WOS Subject | Chemistry, Multidisciplinary |
| WOS ID | WOS:000607831700007 |
| Publisher | HIGHER EDUCATION PRESS |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imr.ac.cn/handle/321006/159030 |
| Collection | 中国科学院金属研究所 |
| Corresponding Author | Fan Xiaolei |
| Affiliation | 1.Univ Manchester, Sch Engn, Dept Chem Engn & Analyt Sci, Manchester M13 9PL, Lancs, England 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 3.Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China |
| Recommended Citation GB/T 7714 | Zou Run,Dong Xiao,Jiao Yilai,et al. Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2021,42(1):74-100. |
| APA | Zou Run,Dong Xiao,Jiao Yilai,D'Agostino, Carmine,Yan Wenfu,&Fan Xiaolei.(2021).Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,42(1),74-100. |
| MLA | Zou Run,et al."Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 42.1(2021):74-100. |
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