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Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites
Zou Run1; Dong Xiao1; Jiao Yilai2; D'Agostino, Carmine1; Yan Wenfu3; Fan Xiaolei1
Corresponding AuthorFan Xiaolei(xiaolei.fan@manchester.ac.uk)
2021-01-10
Source PublicationCHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
ISSN0251-0790
Volume42Issue:1Pages:74-100
AbstractHierarchical zeolites refer to zeolitic materials having bi-/multi-modal interconnective pores arranged in order of certain ranks, which improve the molecular diffusion within their frameworks, and hence the performance in their applications such as adsorption and heterogeneous catalysis. Hierarchical zeolites are commonly produced via the top-down post-synthetic treatments (such as dealumination and/or desilication) of pre-synthesized zeolites (i.e. the parent zeolites) and the bottom-up synthesis-by-design methods (such as soft/ hard templating). This review presents the recent advances (mainly post 2000) in the strategies of making hierarchical zeolites, with the emphasis on the top-down approaches due to their relatively high practicality. Since hierarchical zeolites are proposed to improve intracrystalline diffusion, experimental studies of guest molecules diffusion in hierarchical zeolites are also reviewed. Additionally, catalytic applications of hierarchical zeolites, in comparison with the conventional microporous pristine zeolites, are also commented to highlight the advantages of hierarchical zeolites to improve catalysis.
KeywordHierarchical zeolite Post-synthetic treatment Diffusion Pulsed-field gradient nuclear magnetic resonance( PFG NMR) Catalysis
Funding OrganizationEuropean Union ; China Scholarship Council-The University of Manchester Joint Scholarship ; Programme of Introducing Talents of Discipline to Universities of China ; National Natural Science Foundation of China ; EPSRC New Investigator Award ; Natural Science Foundation of Liaoning Province,China ; National Key Research and Development Program of China
DOI10.7503/cjcu20200461
Indexed BySCI
Language英语
Funding ProjectEuropean Union[872102] ; China Scholarship Council-The University of Manchester Joint Scholarship[201906740020] ; Programme of Introducing Talents of Discipline to Universities of China[B17020] ; National Natural Science Foundation of China[U1967215] ; National Natural Science Foundation of China[21835002] ; National Natural Science Foundation of China[21621001] ; EPSRC New Investigator Award[EP/S019138/1] ; Natural Science Foundation of Liaoning Province,China[2018010047-301] ; National Key Research and Development Program of China[SQ2019YFE011366]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000607831700007
PublisherHIGHER EDUCATION PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/159030
Collection中国科学院金属研究所
Corresponding AuthorFan Xiaolei
Affiliation1.Univ Manchester, Sch Engn, Dept Chem Engn & Analyt Sci, Manchester M13 9PL, Lancs, England
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
3.Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China
Recommended Citation
GB/T 7714
Zou Run,Dong Xiao,Jiao Yilai,et al. Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2021,42(1):74-100.
APA Zou Run,Dong Xiao,Jiao Yilai,D'Agostino, Carmine,Yan Wenfu,&Fan Xiaolei.(2021).Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,42(1),74-100.
MLA Zou Run,et al."Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 42.1(2021):74-100.
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