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Effects of bentonite content on the corrosion evolution of low carbon steel in simulated geological disposal environment
Wei, Xin1; Dong, Junhua1; Chen, Nan2; Yadav, Amar Prasad2,3; Ren, Qiying2; Wei, Jie1; Wang, Changgang1; Ma, Rongyao1; Ke, Wei2
通讯作者Dong, Junhua(jhdong@imr.ac.cn)
2021-03-10
发表期刊JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
ISSN1005-0302
卷号66页码:46-56
摘要The effects of bentonite content on the corrosion behavior of low carbon steel in 5 mM NaHCO3 + 1 mM NaCl + 1 mM Na2SO4 solution were investigated by electrochemical measurements combined with X-ray diffraction (XRD) and scanning electron microscopy (SEM). In the initial immersion stage, the cathodic process of low carbon steel corrosion was dominated by the reduction of dissolved oxygen, while it transformed to the reduction of ferric corrosion products with the immersion time. The presence of bentonite colloids could suppress the cathodic reduction of oxygen due to their barrier effect on the diffusion of oxygen. However, the barrier performance of bentonite layer was gradually deteriorated due to the coagulation and separation of bentonite colloids caused by the charge neutralization of iron corrosion products dissolved from the steel substrate. More bentonite colloids could maintain the barrier effect for a long time before it was deteriorated by the accumulation of corrosion products. Conversely, it could lose the performance completely, and the corrosion behavior of low carbon steel reverted to the same as that in the blank solution. (C) 2021 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
关键词Low carbon steel Bentonite Electrochemical measurements Corrosion products Corrosion evolution
资助者National Natural Science Foundation of China
DOI10.1016/j.jmst.2020.04.071
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[51701222] ; National Natural Science Foundation of China[U1867216 and51471175]
WOS研究方向Materials Science ; Metallurgy & Metallurgical Engineering
WOS类目Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS记录号WOS:000610200200006
出版者JOURNAL MATER SCI TECHNOL
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/159124
专题中国科学院金属研究所
通讯作者Dong, Junhua
作者单位1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China
2.Chinese Acad Sci, Environm Corros Ctr Mat, Inst Met Res, Shenyang 110016, Peoples R China
3.Tribhuvan Univ, Cent Dept Chem, Kathmandu, Nepal
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Wei, Xin,Dong, Junhua,Chen, Nan,et al. Effects of bentonite content on the corrosion evolution of low carbon steel in simulated geological disposal environment[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2021,66:46-56.
APA Wei, Xin.,Dong, Junhua.,Chen, Nan.,Yadav, Amar Prasad.,Ren, Qiying.,...&Ke, Wei.(2021).Effects of bentonite content on the corrosion evolution of low carbon steel in simulated geological disposal environment.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,66,46-56.
MLA Wei, Xin,et al."Effects of bentonite content on the corrosion evolution of low carbon steel in simulated geological disposal environment".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 66(2021):46-56.
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