Stretchable, Stable, and Degradable Silk Fibroin Enabled by Mesoscopic Doping for Finger Motion Triggered Color/Transmittance Adjustment

doi:10.1021/acsnano.1c05257

IMR OpenIR

	Stretchable, Stable, and Degradable Silk Fibroin Enabled by Mesoscopic Doping for Finger Motion Triggered Color/Transmittance Adjustment
	Xu, Zijie 1; Qiu, Wu 2; Fan, Xuwei 3; Shi, Yating 1; Gong, Hao 1; Huang, Jiani 1; Patil, Aniruddha 1; Li, Xuyi 1; Wang, Shutang 1; Lin, Hongbin 1; Hou, Chen 1; Zhao, Jizhong 1; Guo, Xing 4,5; Yang, Yun 1; Lin, Hezhi 3; Huang, Lianfen 3; Liu, Xiang Yang 1,2; Guo, Wenxi 1
通讯作者	Huang, Lianfen(lfhuang@xmu.edu.cn) ; Liu, Xiang Yang(phyliuxy@nus.edu.sg) ; Guo, Wenxi(wxguo@xmu.edu.cn)
	2021-07-27
发表期刊	ACS NANO
ISSN	1936-0851
卷号	15 期号:7 页码:12429-12437
摘要	As a kind of biocompatible material with long history, silk fibroin is one of the ideal platforms for on-skin and implantable electronic devices, especially for self-powered systems. In this work, to solve the intrinsic brittleness as well as poor chemical stability of pure silk fibroin film, mesoscopic doping of regenerated silk fibroin is introduced to promote the secondary structure transformation, resulting in huge improvement in mechanical flexibility (similar to 250% stretchable and 1000 bending cycles) and chemical stability (endure 100 degrees C and 3-11 pH). Based on such doped silk film (SF), a flexible, stretchable and fully bioabsorbable triboelectric nanogenerator (TENG) is developed to harvest biomechanical energy in vitro or in vivo for intelligent wireless communication, for example, such TENG can be attached on the fingers to intelligently control the electrochromic function of rearview mirrors, in which the transmittance can be easily adjusted by changing contact force or area. This robust TENG shows great potential application in intelligent vehicle, smart home and health care systems.
关键词	flexible silk films mesoscopic doping biocompatible triboelectric nanogenerators electronic skin self-power
资助者	National Nature Science Foundation of China ; Shenzhen Basic Research Program ; Natural science foundation of Fujian province ; Fundamental Research Funds for the Central Universities of China ; China Postdoctoral Science Foundation ; 111 Project ; Xiamen University
DOI	10.1021/acsnano.1c05257
收录类别	SCI
语种	英语
资助项目	National Nature Science Foundation of China[51502253] ; National Nature Science Foundation of China[21705135] ; Shenzhen Basic Research Program[JCYJ20180306173007696] ; Natural science foundation of Fujian province[2017J01104] ; Fundamental Research Funds for the Central Universities of China[20720180013] ; China Postdoctoral Science Foundation[2017M612133] ; 111 Project[B16029] ; Xiamen University
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000679406500128
出版者	AMER CHEMICAL SOC
引用统计	被引频次：61[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/159320
专题	中国科学院金属研究所
通讯作者	Huang, Lianfen; Liu, Xiang Yang; Guo, Wenxi
作者单位	1.Xiamen Univ, Coll Phys Sci & Technol, Res Inst Biomimet & Soft Matter, Fujian Prov Key Lab Soft Funct Mat Res, Xiamen 361005, Peoples R China 2.Natl Univ Singapore, Fac Sci, Dept Phys, Singapore 117542, Singapore 3.Xiamen Univ, Coll Informat Sci & Technol, Xiamen 361005, Peoples R China 4.Chinese Acad Sci, Shi Changxu Innovat Ctr Adv Mat, Inst Met Res, Shenyang 110016, Peoples R China 5.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Xu, Zijie,Qiu, Wu,Fan, Xuwei,et al. Stretchable, Stable, and Degradable Silk Fibroin Enabled by Mesoscopic Doping for Finger Motion Triggered Color/Transmittance Adjustment[J]. ACS NANO,2021,15(7):12429-12437.
APA	Xu, Zijie.,Qiu, Wu.,Fan, Xuwei.,Shi, Yating.,Gong, Hao.,...&Guo, Wenxi.(2021).Stretchable, Stable, and Degradable Silk Fibroin Enabled by Mesoscopic Doping for Finger Motion Triggered Color/Transmittance Adjustment.ACS NANO,15(7),12429-12437.
MLA	Xu, Zijie,et al."Stretchable, Stable, and Degradable Silk Fibroin Enabled by Mesoscopic Doping for Finger Motion Triggered Color/Transmittance Adjustment".ACS NANO 15.7(2021):12429-12437.