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Tunable Interaction between Metal-Organic Frameworks and Electroactive Components in Lithium-Sulfur Batteries: Status and Perspectives
Qi, Fulai1; Sun, Zhenhua1,2; Fan, Xialu1,2; Wang, Zhenxing1,2; Shi, Ying1; Hu, Guangjian1; Li, Feng1,2,3
Corresponding AuthorSun, Zhenhua(zhsun@imr.ac.cn) ; Li, Feng(fli@imr.ac.cn)
2021-04-15
Source PublicationADVANCED ENERGY MATERIALS
ISSN1614-6832
Pages25
AbstractLithium-sulfur (Li-S) batteries, with high theoretical energy density, promise to be the optimal candidate of next-generation energy-storage. Rapid development in materials has made a major step forward in Li-S batteries. However, a big gap in cycle life and efficiency for practical applications still remains. Reasonable design of materials/electrodes a is significant aspect that must be addressed. The rising metal-organic frameworks (MOFs) are a new class of crystalline porous organic-inorganic hybrid materials. Abundant inorganic nodes and designable organic linkers allow tailored pore chemistry at a molecular-scale, which enables tunable interaction with electroactive components in Li-S batteries. In this review, the interaction between basic component/structure of MOFs and electroactive components in Li-S batteries is clarified to guide precise function-driven design of MOFs. First, the reaction mechanisms and issues in Li-S batteries are briefly summarized. Second, the structural advantages of MOFs in pore chemistry and morphology are highlighted. Based on the above two aspects of understanding, a bridge between issue-structure-function is proposed. The interaction between MOFs with transport and reaction of electroactive components are discussed. Finally, a perspective on the future development of MOFs based materials in Li-S batteries are given. It is believed that the tunable interaction will boost the frontier interdiscipline of MOFs based electrochemical systems.
Keywordelectroactive components interactions lithium‐ sulfur batteries metal‐ organic frameworks
Funding OrganizationNational Natural Science Foundation of China ; National Key R&D Program of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; LiaoNing Revitalization Talents Program ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Special Projects of the Central Government in Guidance of Local Science and Technology Development ; China Postdoctoral Science Foundation
DOI10.1002/aenm.202100387
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51972313] ; National Natural Science Foundation of China[52020105010] ; National Natural Science Foundation of China[51927803] ; National Natural Science Foundation of China[52072378] ; National Natural Science Foundation of China[51902316] ; National Natural Science Foundation of China[51525206] ; National Key R&D Program of China[2016YFA0200100] ; National Key R&D Program of China[2016YFB0100100] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA22010602] ; LiaoNing Revitalization Talents Program[XLYC1908015] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[Y201942] ; Special Projects of the Central Government in Guidance of Local Science and Technology Development[2020JH6/10500024] ; China Postdoctoral Science Foundation[2019M651162]
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000640240400001
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/162069
Collection中国科学院金属研究所
Corresponding AuthorSun, Zhenhua; Li, Feng
Affiliation1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China
2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China
3.Shenyang Ind Technol Res Inst Energy Mat & Device, Shenyang 110016, Peoples R China
Recommended Citation
GB/T 7714
Qi, Fulai,Sun, Zhenhua,Fan, Xialu,et al. Tunable Interaction between Metal-Organic Frameworks and Electroactive Components in Lithium-Sulfur Batteries: Status and Perspectives[J]. ADVANCED ENERGY MATERIALS,2021:25.
APA Qi, Fulai.,Sun, Zhenhua.,Fan, Xialu.,Wang, Zhenxing.,Shi, Ying.,...&Li, Feng.(2021).Tunable Interaction between Metal-Organic Frameworks and Electroactive Components in Lithium-Sulfur Batteries: Status and Perspectives.ADVANCED ENERGY MATERIALS,25.
MLA Qi, Fulai,et al."Tunable Interaction between Metal-Organic Frameworks and Electroactive Components in Lithium-Sulfur Batteries: Status and Perspectives".ADVANCED ENERGY MATERIALS (2021):25.
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