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Zr含量对Ti-1100合金650℃拉伸变形和断裂机制的影响
其他题名The effect of Zr addition on 650℃deformation and fracture
徐锋
学位类型博士
导师杨锐
2007-08-14
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词高温钛合金 显微组织 硅化物 滑移
摘要本文研究了Zr含量对Ti-1100合金650℃拉伸变形和断裂机制的影响。通过研究发现: 正常Zr含量(4 wt.%)的Ti-1100合金在650℃拉伸变形时:一)合金内存在晶界滑移、位错在α相中的滑移以及α/相界面滑移。其中原始晶粒的晶界滑移是导致合金试样表面起伏不平的主要原因;二)温度升高,位错开动所需临界分切应力减小,在相同的应力条件下可以更容易地观察到柱面滑移,基面滑移和锥面滑移这些不同类型的位错滑移;三)α/β相界面滑移发生在台阶状的{10-10} α // {1-12} β面上并且沿[0002] α //[110]β方向进行;四)α束片层滑移和晶界滑移导致晶界微孔的产生。而β转变组织中α束与晶界α之间关系的差异会产生不同的微孔扩展长大效果。 本文还对正常Zr含量的Ti-1100合金在600℃和650℃拉伸变形和断裂机制的差异进行了研究。结果显示,Ti-1100合金在600℃和650℃拉伸变形时,试样中都存在晶界滑移,穿越α束的位错滑移以及α/β相界面滑移。由于Ti-1100合金的等强温度在600~650℃之间,合金在600℃拉伸断裂时,断口形貌呈现穿晶断裂模式,而在650℃拉伸断裂时,断口形貌呈现沿晶断裂模式。 随合金Zr含量的增加,合金中S2型硅化物的溶解温度升高。当在1050°C进行热加工时,合金处于β+S2两相区,此时合金由β相和S2型硅化物组成。由于S2型硅化物的存在,使β晶界的迁移受阻碍,降低了合金的β晶粒尺寸。当合金进行冷却时,β相中析出晶界α相和α束,与此同时S2型硅化物能够为α相提供非均匀形核的基础,使α相在β晶粒内部能非均匀形核,形成独立α片,这些独立α片之间以及独立α片与α束之间相互交叉,最终形成α束加交叉α片的混合形貌。 合金的显微组织形貌和硅化物的析出规律发生改变,使合金的高温变形和断裂机制也发生相应变化: 首先,α相中硅化物的存在阻碍了位错的长距离滑移,使位错线绕过硅化物前进所需的临界分切应力增加,为了保证合金的进一步变形,位错只能通过交滑移的方式绕过硅化物继续前进;其次,由于原始β晶粒尺寸和α束尺寸的显著下降使得α/β相界面滑移距离也明显下降,同时相互交叉的α片层也会限制α/β相界面的滑移;第三,随合金Zr含量的增加,合金的等强温度升高并超过650℃。当合金在650℃进行拉伸变形时,由于晶界具有较高的强度,晶界滑移造成变形的比例减小,合金的塑性变形主要通过晶内变形来实现,合金的断裂方式由沿晶断裂转变为穿晶断裂。 进一步分析发现,晶界强度是影响合金强度的重要因素。通过增加合金的Zr含量,能强化合金的晶粒和晶界,使合金的等强温度获得提高,导致合金的变形和断裂方式改变,使合金650℃拉伸强度获得显著提高。说明通过提高Zr元素含量的方法,是提高合金的使用温度的一种有效途径。
其他摘要The effects of Zr additions on 650℃ tensile deformation and fracture mechanisms were investigated in Ti-1100 alloy. During 650℃ tensile test for Ti-1100 alloy with 4wt.% Zr, the following results were obtained: 1) grain boundary sliding, long range motion of dislocations in α phase and α/β interface sliding are the main deformation modes; 2) with increase of test temperature, prism slip, basal slip and pyramidal slip were more easily to be observed as a result of decrease of critical shear stress; 3) distinct α/β interface sliding was found to be on {10-10} α // {1-12} β terraces, with sliding direction along [0002] α //[110]β crystal vector ; 4) sliding of α platelet in α colonies and GB α layer leads to creation of mocropores along grain boundary, while orientation relationship difference between α colony and GB α may lead to different extent of micropore propagation . The observation and analyses demonstrate that both lamella sliding and GB sliding control the processes of micropore initiation and intergranular fracture formation. Difference of deformation and fracture mechanisms between 600℃and 650℃tensile tests in Ti-1100 alloy with normal Zr addition was also studied. It was found that Grain boundary sliding, dislocation long range motion in α phase and α/β interface sliding exist in both 600℃and 650℃tensile deformation in Ti-1100 alloy. As the equicohesive temperature of the Ti-1100 alloy is about 600℃, the fracture surface of 600℃tensile sample shows transgranular fracture mode, while the fracture surface of 650℃tensile sample shows intergranular fracture mode. With the increase of Zr content, the dissolution temperature of S2 type silicide increase. If the alloy was heat treated at 1050℃, at this temperature the alloy was in β plus S2 two-phase region. In the subsequent cooling, the silicides were preserved. These residual silicides prevent migration of grain boundary , which result in smaller grain size than Ti-1100 with 4 wt. % Zr. In addition, the residual silicides improve the nohomogeneous nucleation relatively, and result in the transition of the microstructure from lamellar to a mixed one with colony α plus basket weave α morphology. The changes of silicide precipitation process and microstructure lead to changes of deformation and fracture mechanisms at high temperatures: Firstly, the residual silicides block long-range slip of dislocation. Dislocations are unable to round the silicide through Orowan mechanism. In order to continue the deformation process, cross slip of dislocation was necessary; Secondly, decrease of the grain size and colony size shortens the α/β interface sliding distance significantly. Moreover, the basket weave α morphology can also restrict α/β interface slip; Thirdly, with the increase of Zr content, the equicohesive temperatures of the alloys were increased. If the alloys were subjected to tensile tests at 650℃, plastic deformation of the alloys were dominated by deformation within grains because of the strengthened GB and the resultant decrease of deformation from GB sliding. Consequently the fracture mode also changed from intergranular fracture for 1# alloy with normal Zr addition to transgranular fracture for 2#, 3# and 4# alloy with increased Zr addition. These above-mentioned changes of deformation mode and fracture mechanisms lead to increased high-temperature strength. It illustrates that high-temperature tensile properties of Ti-1100 alloy may be improved effectively by increase of Zr content.
页数153
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/16949
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
徐锋. Zr含量对Ti-1100合金650℃拉伸变形和断裂机制的影响[D]. 金属研究所. 中国科学院金属研究所,2007.
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