IMR OpenIR
定向凝固镍基高温合金再结晶行为研究
其他题名Studies on Recrystallization in Directionally Solidified Nickel-base Superalloys
王莉
学位类型博士
导师孙晓峰
2009-05-26
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词镍基高温合金 再结晶 形核 晶粒长大 持久 高温热处理
摘要本论文采用扫描电子显微镜(SEM)、电子背散射衍射技术(EBSD)、电子探针(EPMA)等手段对CMSX-4单晶合金和DZ125L定向凝固柱晶合金的再结晶行为进行了系统研究,分析了再结晶的形核、长大机制。同时研究了合金组织结构特征和外界因素对再结晶行为的影响。并且采用Gleeble热/力模拟试验机对DZ4合金叶片中的再结晶进行了分析、模拟,对DZ4合金及DZ125L合金的再结晶倾向进行了分析。主要内容包括以下几方面: CMSX-4和DZ125L合金经局部变形后,在本论文所选择的温度热处理时(固溶温度附近)都发生了再结晶。较低温度热处理的样品中,只发生部分再结晶;在较高温度热处理时,再结晶进行充分;在远高于固溶温度热处理时,再结晶区域可以观察到较大再结晶晶粒。两种合金的再结晶动力学曲线表明,再结晶过程都是扩散控制的过程。 在不同温度下,再结晶的主要形核机制不同:高温热处理时,枝晶干的再结晶形核是主要形核方式;中温热处理时,可以同时观察到枝晶干形核和枝晶间第二相(碳化物、/¢共晶)和缩孔以颗粒诱发形核机制诱发再结晶形核;而在较低温度热处理时,枝晶间的第二相颗粒诱发再结晶形核为主要形核方式。 在再结晶晶粒长大过程中,组织中的第二相(、/¢共晶、碳化物)与再结晶晶界间的交互作用主要受热处理温度和变形程度的影响。CMSX-4单晶合金中,再结晶晶界受/¢共晶阻碍,可能在/¢共晶内迁移,并在再结晶晶界后析出大块相。DZ125L合金中的碳化物在再结晶晶粒长大过程中阻碍再结晶晶界的迁移。再结晶晶界可以切过或绕过碳化物。当热处理温度较高时,高变形量区的草书体碳化物还有可能在再结晶晶界前沿溶解。 实验发现,在相同变形量、相同热处理制度条件下,随着枝晶间距的增加,再结晶倾向降低;DZ125L合金随碳含量的增加,再结晶倾向性增加,并在碳含量达到0.096 wt%时,再结晶深度达到最大值,继续增加碳含量,再结晶深度变化不大。与DZ125L合金不同,加入300 ppm碳的CMSX-4合金的再结晶倾向明显降低。 观察表层再结晶和局部再结晶在980 oC/235 MPa持久过程中的组织演化发现:(1)表层再结晶在持久过程中变化较小。而(2)局部再结晶在持久过程中的组织变化较为复杂。在垂直于外加拉应力的再结晶晶界上形成了γ′贫化区(PFZ)。持久过程中裂纹产生于PFZ区,PFZ区的产生极有可能是局部再结晶影响合金性能的原因之一。 最后,我们对DZ4叶片中的再结晶进行了观察,研究表明DZ4叶片中的再结晶区一般靠近叶身根部,且面积较大,呈月牙形。叶片中的再结晶区有两种类型,一种是单个或几个大再结晶晶粒构成的再结晶区,另一种是由多个再结晶晶粒构成的再结晶区。分析认为DZ4叶片中的再结晶极有可能是在使用之前就存在的。 对DZ4、DZ125L合金定向凝固、加工、使用过程的热模拟表明:两种叶片在加工、搬运过程中磕碰以及校形时用力不均、变形较大均可导致叶片塑性损伤,从而在随后的高温热处理过程中产生再结晶。
其他摘要Recrystallization (RX) behavior of CMSX-4 and DZ125L alloy was studied by scanning electronic microscope (SEM), electron backscattered diffraction (EBSD) and electron probe microanalyzer (EPMA). RX nucleation mechanisms and grain growth mechanisms were investigated. The effect of microstructure and other factors on RX was analyzed. The RX in DZ4 blades was also observed. Experimental simulation of the RX tendency in DZ4 and DZ125L alloy was also carried out using Gleeble machine. After local indentation and heat treatment at temperatures near the solution temperature, RX took place in all the samples of CMSX-4 and DZ125L. RX occurred partially in the samples heat treated at lower temperature, while full RX occurred at higher temperatures. Large RX grains could be observed when annealed at temperatures much higher than the solution temperature. RX was a diffusion controlled process according to the RX kinetics curves of both alloys. Different RX nucleation mechanisms operate at different temperatures: RX nucleation at dendrite core regions is the dominant nucleation mechanism at high temperatures. Dendrite core nucleation and interdendritic nucleation operate simultaneously at medium high temperature. The interdendritic nucleation was induced by particle (carbides, /¢ eutectics, porosities et. al.) stimulated nucleation (PSN) mechanism. At lower temperatures, RX nucleation by PSN mechanism in interdendritic regions plays an important role. During RX grain growth, the interaction of secondary phase particles (/¢ eutectics, carbides) with RX grain boundary is mainly affected by temperature and deformation. In CMSX-4, RX grain boundary was pinned by /¢ eutectics, or migrated through /¢ eutectics with a large ¢ precipitated behind the boundary. In DZ125L, RX grain boundary was pinned by carbides by different types of interactions: (1) RX grain boundary could cut through or pass by the carbides; (2) in the areas with high level of deformation, scripta-like carbides could be dissolved at the RX grain boundary when annealing at higher temperatures. It was found that less RX happened with increase of primary dendrite arm spacing (PDAS) at the same level of deformation and same process of heat treatment. In DZ125L alloy, RX tendency was increased when the carbon content increased, and a maximum RX depth was observed at 0.096 wt% carbon. Depth of RX didn’t change much with further increase in carbon content. Contrary to that of the DZ125L alloy, less RX occurred when 300 ppm carbon was added to CMSX-4. Microstructure evolution of surface RX and local RX during 980 oC/235 MPa creep test was investigated. It was found that: (1) No obvious change occurred in surface RX. (2) In specimens containing local RX, precipitate free zones (PFZs) were formed during creep along the RX grain boundary that vertical to the applied stress. Crack initiated at PFZ during creep. The detrimental effect of local RX on mechanical properties was probably due to the formation of PFZ. Finally, RX in DZ4 blades was observed. It was found that most of the RX was very large, with the shape of crescent and mainly located at the lower part of the leading and trailing eage, near the root section of the blades. There are two types of RX in the blades, RX areas with single or only several large RX grains and RX areas containing large number of small RX grains. The RX in DZ4 blades was probably happened before service based on the microstructural analysis. Based on the results obtained from Gleeble simulation of the directional solidification (DS) process, machining and service, it can be concluded that plastic deformation could be induced during processing of the blade, and RX could be induced during the following high temperature annealing.
页数106
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17047
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
王莉. 定向凝固镍基高温合金再结晶行为研究[D]. 金属研究所. 中国科学院金属研究所,2009.
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