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铼和钴在单晶高温合金中的作用
其他题名Wenzhen Wang
王文珍
学位类型博士
导师胡壮麒
2008-01-25
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词 粗化 Tcp相 单晶高温合金
摘要本文研究了合金元素铼(Re)和钴(Co)对单晶高温合金组织和性能的影响及二者之间的交互作用,结果表明: 随着Re含量的升高,铸态相的尺寸减小,合金的初熔温度提高,共晶的溶解和偏析的消除变得困难,获得形状规则、尺寸适中的的一次时效温度升高;Re含量增加,扩散系数降低,抑制了粗化;Re有利于提高合金的持久性能。 随着Co含量的升高,铸态相体积分数升高,尺寸减小,合金的初熔温度降低,共晶的溶解和偏析的消除变得容易;Co含量增加,扩散系数升高,促进了粗化,抑制了TCP相的析出;Co提高了无Re合金的持久性能,不降低含Re合金的性能,在Re含量较高的合金中,可以通过适当增加Co含量来抑制有害相的析出。 Co对变形机制的影响在含Re合金和无Re合金中不同。含Re合金在850℃/586MPa持久条件下,含12wt.%Co的合金中位错切入形成层错。无Re合金在1010℃/248MPa持久条件下:含12wt.%Co的合金中位错切入形成反相畴;不含Co的合金中位错切入形成层错。位错切入形成层错还是反相畴取决于Re和Co对层错能和反相畴界能的共同影响。 在950℃和1050℃长期时效后,为立方形、球形或不规则形状时,长期时效过程中其粗化更多地受扩散控制;为筏形时,其粗化更多地受界面反应控制。提出了一个描述形筏过程的模型。 研制出了一种含4wt.%Re、12wt.%Co的新型低成本第三代单晶高温合金,其持久寿命与含6wt.%Re的国外第三代单晶合金相当,且具有较高的抗拉强度、良好的抗氧化、抗热腐蚀性能以及优异的长期时效组织稳定性。
其他摘要In this dissertation, the effects of Rhenium (Re) and Cobalt (Co) on the microstructures and properties and the interactions between them in single crystal superalloys are investigated. With the increasing of rhenium content, the size of as-cast  reduces and the incipient melting points of alloys enhance. With the rising of rhenium content, the dissolution of eutectics and the alleviation of chemical segregation becomes more difficult. When the content of Re is rising, the primary ageing temperature heightens. With the increasing of rhenium content, the diffusion coefficient reduces and  coarsening is inhibited. Re is beneficial to improve the creep rupture lives. With the increasing of cobalt content, the volume fraction of as-cast  increases and the size of  decreases. When the content of Co is rising, the incipient melting points of alloys lower. With the the increasing of Co content, the dissolution of eutectics and the alleviation of chemical segregation becomes easier. With the the rising of Co content, the diffusion coefficient elevates, which accelerates  coarsening and suppresses the formation of TCP phase. With the increasing of cobalt content, the creep rupture lives of alloys free of Re improve and that of alloys containing Re do not degrade. In alloys containing high levels of Re, the deleterious phases can be eliminated by adding some contents of cobalt. The influences of cobalt on deformation mechanisms in Re-containing alloys are quite different from that in the alloys free of Re. For the alloys containing Re, the  particles are cut by stacking faults (SF) in the alloy having 12wt.% Co when creep ruptured at 850℃/586MPa. However, for the alloys free of Re, when they creep ruptured at 1010℃/248MPa, the  particles are cut by dislocation pairs coupled with APB in the alloy containing 12wt.%Co, while the  particles are cut by stacking faults in the alloy free of Co. The cutting of  particles by stacking faults or by dislocation pairs coupled with APB depends on the interactions of Re and Co on the energies of SF and APB. After long-term ageing at 950℃ and 1050℃, when  was cubic, global or irregular, its coarsening is more controlled by diffusion; when  formed rafts, its coarsening is more controlled by interface reaction. A model of describing the process of forming rafts is established. In this dissertation, a low cost third generation single crystal superalloy containing 4wt.% Re and 12wt.%Co is developed. The creep rupture lives of this alloy approach or achieve the levels of alien third generation single crystal superalloys having 6wt.% Re. This alloy has also high tensile strength, good oxidation and hot corrosion resistance properties, excellent microstructural stabilities and high strength after long time exposure.
页数112
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17049
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
王文珍. 铼和钴在单晶高温合金中的作用[D]. 金属研究所. 中国科学院金属研究所,2008.
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