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冷喷涂制备TiAl3-Al复合涂层及抗氧化性能研究
其他题名INVESTIGATION ON COLD GAS DYNAMIC SPRAYED TiAl3-Al COMPOSITE COATING AND ITS OXIDATION RESISTANCE
沈莉
学位类型硕士
导师熊天英
2008-05-29
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料加工工程
关键词冷喷涂 钛/铝复合涂层 Tial3-al复合涂层 力学性能 抗高温氧化
摘要本实验采用冷喷涂的方法将钛粉和铝粉按原子比1:3混合后在多元Ti2AlNb型合金基体上成功沉积钛/铝(Ti/Al)复合涂层,通过对冷喷涂过程的主要工艺参数进行正交实验设计,以涂层的密度作为评价标准,获得了致密性最佳的涂层,喷涂工艺参数为:喷涂距离为10 mm,载气温度为250 ℃,载气压力为1.8 MPa。随后在高纯氩气保护气氛中对钛/铝复合涂层进行合金化热处理(加热温度630 ℃,保温5 h的,升温速率为3 ℃/min,氩气流量为40 ml/min),得到TiAl3-Al复合涂层。利用XRD,SEM和EDS分析手段研究了涂层的微观结构和相组成,分别利用图像分析软件和力学设备测定了涂层孔隙率、显微硬度和结合强度。随后对带涂层TiAl3-Al和不带涂层的 Ti2AlNb型多元合金Ti751基体进行了高温氧化行为研究。研究结果表明,在 950 ℃空气中恒温氧化100小时后,仅有Ti751基体的样品表面形成了疏松多孔的氧化膜,氧化膜大面积脱落,氧化膜以TiO2为主,还有少量的AlNbO4和Al2O3,该样品的氧化曲线近似呈线性增加的趋势;带有TiAl3-Al涂层的样品动力学曲线符合抛物线规律,涂层表面形成了致密的氧化膜,且仍与基体结合良好。与仅有Ti751基体的样品相比,带有TiAl3-Al涂层的样品在950 ℃空气中恒温氧化100 h的过程中增重较少,不带涂层样品的增重是带涂层样品的7倍,表明TiAl3-Al涂层具有良好的抗氧化性能。
其他摘要A kind of composite coating using mixed powder of pure aluminum and pure titanium as feedstock was successfully deposited on orthorhombic Ti2AlNb alloy substrate by cold gas dynamic spraying. The ratio of pure titanium to pure aluminum of the powder was fixed at 1:3 in atom. The best parameters of the cold gas dynamic spraying experiment were obtained from analyzing the orthogonal table of spraying parameters when the density of coating was as evaluation criterion. The as-sprayed composite coating was heat-treated at 630 ℃ in flowing argon atmosphere for 5 h. The heating rate was controlled at 3 ℃/min and the flowing rate of the argon gas was kept at 40 ml/min. Analysis and characterization of sprayed and heat-treated coating were performed by means of scanning electron microscopy with EDS and image analysis system. X-ray diffraction was employed to investigate the structure changes between as-sprayed and heat-treated coatings. The coating’s mechanical properties, including micro-hardness and bonding strength were analyzed as well. It was found that the composite coating of the intermetallic compound TiAl3 and Al was formed and performed good bonding with the substrate after alloying heat treatment. The isothermal oxidation behaviors of orthorhombic Ti2AlNb complex alloy Ti751 and the alloy with TiAl3-Al coating was studied respectively at 950 ℃ in static air. The results indicated that oxidation kinetic curve of the Ti751 substrate with TiAl3-Al coatings was according to the parabolic law, and the surface oxide scale kept almost invariant and no crack was found at the interface of coating and substrate. The oxidation kinetic curve of Ti751 alloy substrate was increasing linearly, and the surface oxide scales were loose and porous, they are mostly TiO2 and little AlNbO4, and Al2O3. The high temperature oxidation resistance of the Ti2AlNb complex alloy Ti751 substrate with TiAl3-Al coatings was much higher than that of the naked substrate.
页数73
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17197
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
沈莉. 冷喷涂制备TiAl3-Al复合涂层及抗氧化性能研究[D]. 金属研究所. 中国科学院金属研究所,2008.
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