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Ti-60A合金中的硅化物及原始β晶粒尺寸控制研究
其他题名Study on Silicide of Ti-60A High-Temperature Titanium Alloy and Control of β Grain Size
赵亮
学位类型硕士
导师杨锐
2008-05-27
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词高温钛合金 Ti-60a 硅化物 高温蠕变 持久 晶粒度 尺寸分布
摘要高温钛合金由于具有密度低,比强度高,高温性能好等优点而广泛应用于航空航天领域。Ti-60A合金属于Ti-Al-Zr-Mo-Si-Sn系近α型高温钛合金,使用温度已经达到600℃。影响高温钛合金性能的因素很多,Ti-60A合金中的硅化物和β晶粒尺寸控制是目前研究尚不充分的两个方面。因此,本文研究了Ti-60A合金中硅化物的析出、溶解温度,硅化物析出的位置、形貌和尺寸,并研究了不同条件下硅化物析出对Ti-60A合金高温蠕变和持久性能的影响;最后研究了热处理和热加工工艺对Ti-60A合金原始β晶粒尺寸及分布的影响。 实验结果表明,Ti-60A合金中硅化物的析出温度为990℃,完全溶解温度为1030℃,850℃左右硅化物析出量最多,尺寸从几十到几百纳米不等, 600℃以下硅化物析出量较少,尺寸通常小于100纳米。硅化物析出的形状多样,900℃以上以纺锤状为主,且硅化物与基体界面不明显,900℃~800℃以多面体形状为主,750℃以下多为短棒状。硅化物的析出,与基体有一定的取向关系,在本文实验中观察的硅化物与α相基体的取向关系为:硅化物[0001]晶带轴平行于基体[123(__)1]晶带轴,硅化物(1(__)21(__)0)面平行于基体(01(__)12) 面。 在外加应力水平较低的蠕变实验条件下,材料变形以界面为主,硅化物在α片层之间析出,对α片层界面起到有效的钉扎作用,提高材料蠕变抗力。在外加应力水平较高的持久实验条件下,Ti-60A钛合金中硅化物的大量析出降低了材料的持久性能。在此条件下,选择硅化物少量析出但α2析出明显的热处理工艺对提高持久性能有利。在高温大应力持久实验条件下,位错在大颗粒硅化物处产生塞积,导致硅化物开裂或与基体脱粘产生微孔,微孔聚集后发生过早断裂是导致持久性能降低的主要原因。 α2相的析出对提高Ti-60A钛合金的蠕变抗力和持久断裂时间都是有利的,但硅化物的析出只对提高蠕变性能有利,对持久性能的作用取决于硅化物的析出量及颗粒尺寸。Ti-60合金的蠕变性能和持久性能不一定同时达到最佳。 Ti-60A合金棒材中的原始β晶粒尺寸呈正态分布。原始坯料显微组织比较粗大时,较大的锻造变形量会改善Ti-60A合金棒材原始β晶粒尺寸均匀性;当锻造变形量达到33%时,Ti-60A合金棒材原始β晶粒尺寸变小,均匀性得到进一步改善;Ti-60A合金在α+β相区轧制,变形量达到40%以上时,坯料的原始显微组织对原始β晶粒尺寸均匀性及颗粒平均尺寸的影响不大;轧制加热温度在α+β相区时,轧制温度升高会使原始β晶粒尺寸分布曲线向尺寸较大的方向移动。
其他摘要High temperature titanium alloys have been used widely in aerospace because of the low density, specific strength and good performance at high temperature. Ti-60A alloy which is belong to Ti-Al-Zr-Mo-Si-Sn alloy system is a near-α high temperature titanium alloy. It can be used stably up to 600℃. Silicide and β grain size are two important factors in Ti-60A alloy, which are not studied sufficiently yet. Therefore, this thesis focused on silicide precipitation and solution temperature, precipitation position, shape, and size. Furthermore, the thesis studied the effect of silicide precipitation on high temperature creep and creep rupture behavior. At last the thesis explored how to control β grain size and distribution in Ti-60A alloy. Microstructure analysis by TEM showed that silicide precipitation begins at 990℃, and solution completely at 1030℃, under 2 hours annealing. The most precipitation appears at about 850℃. The silicide size is about tens nanometers to hundreds nanometers. Silicide precipitation had a small quantity and less than 100 nanometers When the annealing temperature below 600℃.Annealing at 900℃, silicide is spindle, and has indistinct boundary with the matrix. At 900℃~800℃, silicide precipitated as polyhedral. Below 750℃, silicide looks like short stick. Silicide had orientation relationship with the α phase matrix: [0001] S2∥[123(__)1] α, (1(__)21(__)0) S2∥(01(__)12) α. Silicide precipitation between α plates anchored α and β phase interface, when the creep stress is low, so it can improve the creep resistance at 600℃and this effect become more pronounced when α2 phase precipitated in the matrix. However, when the creep stress is high, the effect of silicide on the creep rupture property was negative. Because of the silicide precipitation, dislocation tangled near the silicide, then, cracks initiated from the tangled dislocation. Precipitation of α2 phase was beneficial both to high temperature creep and creep rupture properties. Increase of silicide in solution by way of lowering the silicide precipitation was concluded to be more beneficial to creep rupture properties with higher applied stress than to creep properties with lower applied stress. Different grain size and grain distribution of primary β grains could be achieved by controlling the deformation rate and temperature of precision forging and hot rolling. We found that the effects of the thermomechanical processing on grain size and distribution were minor when Ti-60A was heat treated near the α+β/β transformation temperature, while it was heat treated above the α+β/β transformation temperature, the differences of the grain size and distribution of all the samples were disappeared.
页数60
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17208
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
赵亮. Ti-60A合金中的硅化物及原始β晶粒尺寸控制研究[D]. 金属研究所. 中国科学院金属研究所,2008.
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