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Bulk growth and separation of single-walled carbon nanotubes from rhenium catalyst
Ma, Chen1; Liu, Yumin2; Zhang, Lili3; Qian, Liu4; Zhao, Yiming3; Tian, Ying5; Wu, Qianru1; Li, Dong1; Zhao, Nan1; Zhang, Xueting1; Xin, Liantao1; Liu, Huaping2; Hou, Pengxiang3; Liu, Chang3; He, Maoshuai1; Zhang, Jin4
Corresponding AuthorLiu, Huaping(liuhuaping@iphy.ac.cn) ; He, Maoshuai(hemaoshuai@qust.edu.cn) ; Zhang, Jin(jinzhang@pku.edu.cn)
2022-04-08
Source PublicationNANO RESEARCH
ISSN1998-0124
Pages6
AbstractBulk synthesis of single-walled carbon nanotubes (SWNTs) using solid catalyst has been challenging, despite of recent breakthrough in the chirality-specific growth on the flat substrate surface. In this work, we propose a porous magnesia support rhenium catalyst for bulk synthesis of SWNTs. It is found that the well-dispersed catalyst with a high melting point and the optimal chemical vapor deposition reaction conditions account for the growth of SWNTs. Detailed characterizations reveal the produced SWNTs are dominant in (n, n - 1) and (n, n - 2) species. Furthermore, by using a multicolumn chromatography post-growth separation method, SWNTs with three defined diameter ranges were obtained. This work guides the design of porous oxide supported catalyst for bulk synthesis and diameter-dependent sorting of SWNTs, which will ultimately help harness the extraordinary properties of SWNTs.
Keywordsingle-walled carbon nanotube rhenium catalyst bulk growth gel chromatography diameter separation
Funding OrganizationNational Key Research and Development Program of China ; National Natural Science Foundation of China ; Key Basic Research Project of Shandong Province ; Strategic Priority Research Program of Chinese Academy of Sciences ; Key Research Program of Frontier Sciences, CAS ; Youth Innovation Promotion Association of CAS ; Taishan Scholar Advantage and Characteristic Discipline Team of Eco Chemical Process and Technology
DOI10.1007/s12274-022-4248-z
Indexed BySCI
Language英语
Funding ProjectNational Key Research and Development Program of China[2020YFA0714700] ; National Key Research and Development Program of China[2018YFA0208402] ; National Natural Science Foundation of China[51972184] ; National Natural Science Foundation of China[51820105002] ; National Natural Science Foundation of China[11634014] ; National Natural Science Foundation of China[51872320] ; Key Basic Research Project of Shandong Province[ZR2019ZD49] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB33030100] ; Key Research Program of Frontier Sciences, CAS[QYZDBSSW-SYS028] ; Youth Innovation Promotion Association of CAS[2020005] ; Taishan Scholar Advantage and Characteristic Discipline Team of Eco Chemical Process and Technology
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000782173200003
PublisherTSINGHUA UNIV PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/172786
Collection中国科学院金属研究所
Corresponding AuthorLiu, Huaping; He, Maoshuai; Zhang, Jin
Affiliation1.Qingdao Univ Sci & Technol, Taishan Scholar Adv & Characterist Discipline Tea, State Key Lab Ecochem Engn, Minist Educ,Coll Chem & Mol Engn, Qingdao 266042, Peoples R China
2.Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China
4.Peking Univ, Beijing Sci & Engn Ctr Nanocarbons, Coll Chem & Mol Engn, Ctr Nanochem,Beijing Natl Lab Mol Sci,Coll Chem &, Beijing 100871, Peoples R China
5.Dalian Maritime Univ, Sch Sci, Dalian 116026, Peoples R China
Recommended Citation
GB/T 7714
Ma, Chen,Liu, Yumin,Zhang, Lili,et al. Bulk growth and separation of single-walled carbon nanotubes from rhenium catalyst[J]. NANO RESEARCH,2022:6.
APA Ma, Chen.,Liu, Yumin.,Zhang, Lili.,Qian, Liu.,Zhao, Yiming.,...&Zhang, Jin.(2022).Bulk growth and separation of single-walled carbon nanotubes from rhenium catalyst.NANO RESEARCH,6.
MLA Ma, Chen,et al."Bulk growth and separation of single-walled carbon nanotubes from rhenium catalyst".NANO RESEARCH (2022):6.
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