Large-Scale Epitaxial Growth of Ultralong Stripe BiFeO3 Films and Anisotropic Optical Properties

doi:10.1021/acsami.1c22248

IMR OpenIR

	Large-Scale Epitaxial Growth of Ultralong Stripe BiFeO3 Films and Anisotropic Optical Properties
	Wang, Han 1,2; Wu, Haijun 1,3; Chi, Xiao 4; Li, Yangyang 1; Zhou, Chenghang 1; Yang, Ping 4; Yu, Xiaojiang 4; Wang, John 1; Chow, Gan-Moog 1; Yan, Xiaobing 5; Pennycook, Stephen John 1; Chen, Jingsheng 1
通讯作者	Chen, Jingsheng(msecj@nus.edu.sg)
	2022-02-16
发表期刊	ACS APPLIED MATERIALS & INTERFACES
ISSN	1944-8244
卷号	14 期号:6 页码:8557-8564
摘要	The controlled synthesis of large-scale ferroelectric domains with high uniformity is crucial for practical applications in next-generation nanoelectronics on the basis of their intriguing properties. Here, ultralong and highly uniform stripe domains in (110)-oriented BiFeO3 thin films are large-area synthesized through a pulsed laser deposition technique. Utilizing scanning transmission electron microscopy and piezoresponse force microscopy, we verified that the ferroelectric domains have one-dimensional 109 degrees domains and the length of a domain is up to centimeter scale. More importantly, the ferroelectric displacement is directly determined on atomic-scale precision, further confirming the domain structure. We find that the unique one-dimensional ferroelectric domain significantly enhances the optical anisotropy. Furthermore, we demonstrate that the purely parallel domain patterns can be used to control photovoltaic current. These ultralong ferroelectric domains can be patterned into various functional devices, which may inspire research efforts to explore their properties and various applications.
关键词	ferroelectric stripe domain self-assembly optical anisotropy (110) BiFeO3 X-ray absorption spectroscopy
资助者	A*STAR ; Singapore Ministry of Education ; National Natural Science Foundation of China ; Young Talent Program of SYNL
DOI	10.1021/acsami.1c22248
收录类别	SCI
语种	英语
资助项目	ASTAR[A1983C0036, ASTAR IAF-ICP 11801E0036] ; Singapore Ministry of Education[MOE2018-T2-1-019] ; Singapore Ministry of Education[MOE2018-T2-2-043] ; Singapore Ministry of Education[MOE Tier1 R-284-000-195-114] ; Singapore Ministry of Education[MOE Tier1 R-284-000-196-114] ; National Natural Science Foundation of China[61674050] ; National Natural Science Foundation of China[61874158] ; Young Talent Program of SYNL
WOS研究方向	Science & Technology - Other Topics ; Materials Science
WOS类目	Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000769573400101
出版者	AMER CHEMICAL SOC
引用统计
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/173105
专题	中国科学院金属研究所
通讯作者	Chen, Jingsheng
作者单位	1.Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117575, Singapore 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 3.Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China 4.Natl Univ Singapore, Singapore Synchrotron Light Source SSLS, Singapore 117603, Singapore 5.Hebei Univ, Coll Electron & Informat Engn, Baoding 071002, Peoples R China
推荐引用方式 GB/T 7714	Wang, Han,Wu, Haijun,Chi, Xiao,et al. Large-Scale Epitaxial Growth of Ultralong Stripe BiFeO3 Films and Anisotropic Optical Properties[J]. ACS APPLIED MATERIALS & INTERFACES,2022,14(6):8557-8564.
APA	Wang, Han.,Wu, Haijun.,Chi, Xiao.,Li, Yangyang.,Zhou, Chenghang.,...&Chen, Jingsheng.(2022).Large-Scale Epitaxial Growth of Ultralong Stripe BiFeO3 Films and Anisotropic Optical Properties.ACS APPLIED MATERIALS & INTERFACES,14(6),8557-8564.
MLA	Wang, Han,et al."Large-Scale Epitaxial Growth of Ultralong Stripe BiFeO3 Films and Anisotropic Optical Properties".ACS APPLIED MATERIALS & INTERFACES 14.6(2022):8557-8564.