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Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties
Li, Zhenyu1,2; Zhao, Linmin3; Chen, Hui1; Liang, Xiao1; Ai, Xuan1; Xie, Zhoubing1; Li, Xiaotian2; Yang, Feng4; Liu, Hongyang3; Zou, Xiaoxin1
Corresponding AuthorLiu, Hongyang(liuhy@imr.ac.cn) ; Zou, Xiaoxin(xxzou@jlu.edu.cn)
2021-12-13
Source PublicationCATALYSIS SCIENCE & TECHNOLOGY
ISSN2044-4753
Pages5
AbstractThree crystal phases of Pd-B intermetallics, namely, Pd6B, Pd5B2 and Pd2B, are synthesized, and their phase-dependent catalytic activities toward electrochemical water splitting and Suzuki coupling reactions are studied. In both reactions, their catalytic activities are found to increase in the order Pd, Pd6B, Pd5B2 and Pd2B. This activity trend is strongly associated with the Pd(d)-B(s,p) orbital hybridization-regulated surface adsorption properties.
Funding OrganizationNational Natural Science Foundation of China (NSFC) ; Fok Ying Tung Education Foundation ; Fundamental Research Funds for the Central Universities, NSFC ; 111 Project
DOI10.1039/d1cy02112e
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China (NSFC)[21922507] ; National Natural Science Foundation of China (NSFC)[21771079] ; National Natural Science Foundation of China (NSFC)[21901083] ; National Natural Science Foundation of China (NSFC)[22179046] ; Fok Ying Tung Education Foundation[161011] ; Fundamental Research Funds for the Central Universities, NSFC[21621001] ; 111 Project[B17020]
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000747885300001
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/173618
Collection中国科学院金属研究所
Corresponding AuthorLiu, Hongyang; Zou, Xiaoxin
Affiliation1.Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China
2.Jilin Univ, Coll Mat Sci & Engn, Changchun 130022, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
4.Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China
Recommended Citation
GB/T 7714
Li, Zhenyu,Zhao, Linmin,Chen, Hui,et al. Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties[J]. CATALYSIS SCIENCE & TECHNOLOGY,2021:5.
APA Li, Zhenyu.,Zhao, Linmin.,Chen, Hui.,Liang, Xiao.,Ai, Xuan.,...&Zou, Xiaoxin.(2021).Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties.CATALYSIS SCIENCE & TECHNOLOGY,5.
MLA Li, Zhenyu,et al."Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties".CATALYSIS SCIENCE & TECHNOLOGY (2021):5.
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