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稀土元素改性反应离子镀涂层的结构和性能
刘长清
学位类型硕士
导师吴维安
1988
学位授予单位中国科学院金属腐蚀与防护研究所
学位授予地点中国科学院金属腐蚀与防护研究所
摘要通过分段离子镀的偿试。获得了如下含稀土元素Y的复合涂层。TiN/Y, Ti/Y, TiN/Ti/Y, Ti(R)N/Ti(R)/Y; TiN/YN/Y Ti(R)N/YN/Y; Ti(R)N/Ti(R)/Ti; ((R)表示镀膜过程使用Ti-Y合金作蒸发源)。以EPMA、IMA、AES、XRD等分析手段研究涂层的元素分布和相分布。发现所有含稀土Y涂层中Y元素富集于界面附近。Ti(R)N涂层界面区Y含量约为(0.2 ~ 0.5)%, Wt。各涂层中的相组成及择优取向有所差别。Ti(R)N涂层具有明显的密排面(lll)晶面的强衍射峰,而TiN则具有(200)晶面强衍射峰。划痕法和动态拉伸法评定涂层结合强度表明。Ti(R)N/Ti(R)/Ti涂层界面结合最为优良。Ti(R)N涂层结合强度优于TiN涂层。而Ti(R)涂层界面结合不如Ti涂层。通过测定涂层在几种介质中的极化曲线认为。离子镀Ti耐蚀性优于蒸镀Ti主要是在前一种情况下对试样加负偏压使涂层更为致密和均布所致。极图分析Ti(R)N及TiN涂层表明,Ti(R)N涂层具有(112)主要面积织构,TiN则有(110)主要面织构,这可能成为Ti(R)N涂层耐蚀性优于TiN涂层的主要原因之一。此外,通过Ti(R)N涂层镀膜过程中的熔料分析证明了。稀土Y界面富集机制是:优先蒸发和微扩散,还讨论涂层在外加载荷作用下破坏的可能机制。
其他摘要Through multisteps plating technique, various ion plated or reactive ion plated coatings were obtained in the laboratory. They are as follows: TiN/Y, Ti/Y, TiN/Ti/Y, Ti(R)N/Ti(R)/Y, TiN/YN/Y, Ti(R)N/YN/Y, Ti(R)N/Ti(R)/Ti, (here (R) presents the use of Y-containing Ti-alloy as evapouration source). By means of EPMA, IMA, AES, XRD, etc. Element and phase distribution in the coatings was studied. It was found that rear-earth Y in the coatings is concentrated at the coating/substrate interface. Y content at the interface area of Ti(R)N coating was about (0.2 - 0.5)wt%. The type and amount of the phases and the preferred orientations of the crystallites of the coatings were different. The Ti(R)N coating showed preferred orientation of TiN(lll) parallel to the sample surface, while the TiN coating had preferred orientation of TiN(200). The coating/substrate adhesive evaluated by scratch test and constant pulling rate tensile test showed that Ti(R)N coating was better than TiN coating without Y, However, Ti(R) coating is poorer than Ti coating through measuring the polarization curves of the coatings in several sorts of corrosion medium, it is obvious that IP-Ti coating has better corrosion-resistance than VP-Ti coating which may be due to negative bias which enable the IP-Ti coating becoming of higher degree of compactness and uniformity, pole figures of Ti(R)N and TiN coating show that Ti(R)N coating has main texture of TiN(112), TiN coating has TiN(110), that may be the main reason for better corrosion-resistance of Ti(R)N coating. Comparing the results of element profiles of the coating and the analysis of the change of alloying content at the top surface area of the evaporation source with evaporation time, one can proposed the enrichment of rare earth element Y at the interface may due to its selected evaporation and diffusion via some short circuits. Additionaly, the possible damage mechanism of TiN type coating under loading was also proposed.
页数136
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17370
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
刘长清. 稀土元素改性反应离子镀涂层的结构和性能[D]. 中国科学院金属腐蚀与防护研究所. 中国科学院金属腐蚀与防护研究所,1988.
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