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刷镀—复合镀的研究
曹礼群
学位类型硕士
导师姜晓霞
2001
学位授予单位中国科学院金属研究所
学位授予地点中国科学院金属研究所
摘要以Ni-SiO_2、Cu-Al_2O_3两个体系为主,通过测定镀层中粒子含量,镀层硬度及耐磨性等,系统研究了复合刷镀的各工艺参数对镀层形成及性能的影响,找出了复合刷镀的最佳工艺条件。同时证实用石墨镀笔得到的镀层严格地讲都是复合镀层。为了扩大刷镀范围还试验并刷镀成功了Ni-Al_2O_3、Ni-P-BaF_2、Cu-BC、Cu-SiO_2等几个体系。只有保持粒子在镀液中悬浮和分散才有利于形成刷镀一复合镀层,表面活性剂对粒子悬浮具有重要意义。本文研究了它对粒子的悬浮的影响,并找到了Ni-SiO_2、Cu-Al_2O_3的有效配方。分析变为表面活性剂作用是通过吸附形成界面膜,降低体系能量,增加粒子表面电荷,提高溶液粘度等途径实现的。测定溶液电位,极化曲线,交流阻抗等结果表明表面活性剂在粒子及电极表面上吸附,但未发现它对镀层性能有明显影响。对刷镀一复合镀过程进行了探讨,还比较讨论了槽镀复合镀(电镀、化学镀)与刷镀复合镀的异同。实验结果表明刷镀中阴阳极相对运动速度和粒子特性是得到刷镀一复合镀层的关键。刷镀对粒子的嵌合能力远小于槽镀。
其他摘要The effect of the technical parameters in composite brush electroplating on the deposition and the properties of coating such as the content of particles, microhardness and wear resistance had been investigated in Ni/SiO_2 and Cu/Al_2O_3 system. The optimal operation and variables were obtained. The experiment showed that the common brush electroplating using the graphite anode prepared the metal/graphite composite coating acturally. In present work it was also successful to brush the composite coating of Ni-P/BaF_2, Cu/BC, Ni/Al_2O_3 and Cu/SiO_2 etc.. The key of formation of the brush composite coating was the suspension and dispersion of particles in plating solution continuously. The surfactant in solution plays an important role in suspension and dispersion of particles. The influence of surfactant on suspension of particle was studied in this work and how to prepare the brush plating solution of Cu/Al_2O_3 and Ni/SiO_2 was developed. It has been deduced that the surfactant could form the adsorption film on the interface, decrease the energy of the system, increase the surface charge of particles and raise the viscosity of plating solution. The adsorption of surfactant on the surface of particles and electrode was proven by the potential change, polarization curve and AC impedance. No obvious influence on the properties of coating was observed. The process of brush electroplating and the difference between brush and bath plating (electro and electroless plating) were discussed. The results of experiments show that the speed of relative movement of anode and cathode, the character of particles are two important parameters in brush plating of composite coating. The composite ability of particles in brush plating is less than that in bath (electro and electroless) plating.
页数83
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17447
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
曹礼群. 刷镀—复合镀的研究[D]. 中国科学院金属研究所. 中国科学院金属研究所,2001.
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