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动态离子束混合对金属腐蚀和疲劳行为的影响
陈自力
学位类型硕士
导师金属物理
1990
学位授予单位中国科学院金属研究所
学位授予地点中国科学院金属研究所
摘要本文使用AES、XRD、TEM研究了多晶镍动态离子束混合钛、氮化铬后表面层组成和微观结构,同时研究其弯化对腐蚀行为影响的机制。另外还研究了多晶镍动态混合钛对其疲劳行为的影响。研究结果表明,动态混合钛、氮化铬改性层中只有部分沉和积层与基体镍发生混合。但由于Ni在Ti中超常扩散,使钛混合区增宽,且镍已扩散到表面。混合过程中碳污染与沉积原子反应生碳化物。动态混合钛、氮化铬后由表面到基底形成一个不同组织结构的多层次的混合层,钛混合层由氧化物,织构α-Ti、TiC、Ti_2NiHo.5和位错胞结构组成;氮化铬混合层由Cr-N-C非晶,Cr_2(CN)、Cr(b.c.c.)、Cr(Cubic),Ni-Cr非晶和位错胞结构组成。多晶镍动态混合钛、氮化铬使其耐腐蚀性能得到极度大提高,临界腐蚀电流和钝化电流密度分别降低两和一个量级,且后者持久耐蚀性好于前者。前者提高原因归结于表面氧化膜,后者归结于表面Cr-N-C非晶层。且前者耐点蚀能力也得到增强。多晶镍混合钛、氮化铬后提高了其表面硬度。在应力控制拉-零疲劳条件下,多晶镍动态混合钛使其疲劳寿命降低。降低原因归结于表面层在循环应力作用下塑性开裂,使疲劳裂纹萌生时间缩短和疲劳裂纹增多。
其他摘要In this paper, titanium and chromium nitride coatings on pure polycrystalline nickel wee obtained by dynamic ion beam mixing. Chemical composition and microstructure of the surface layers were examined by AES, XRD, TEM, and their effects on corrosive properties as well Ti-DIBM specimen fatigue behaviour were studied. Composition analyses by AES show that only the part of condensing layers is mixed with the substrates. Because nickel exhibits ultra-fast solut diffusion in α-Ti, the mixed profile extends to surface. TEM analyses show that the Ti-DIBM specimen surface region consists of titanium oxide, collum grown α-Ti, TiC, Ti_2NiHo.5 phases and the cell structure of dislocations; The CrN-DIBM specimen surface region consists of Cr-N-C amorphous, Cr_2(CN), Cr(b.c.c), Cr(cubic), Ni-Cr amorphous phases and the cell structure of dislocations. The three-sweep potentiokinetic measureent of the specimens in deaerated 1M NaAc/HAC (PH6.7, 25 ℃) shows that corrosion resistance is improved significantly. The critical current density and the minimum anodic passivating current density are lowered by about one or two orders of magnitude, respectively, and the latter is better than the former. Ti-DIBM specimen corrosion resistance improvement is attributed to the oxide surface layer. Ti-DIBM specimen corrosion resistance improvement is attriuted to the oxide surface layer. CrN-DIBM specimen corrosion resistance imporovment is attributed to the amorphous surface layer. The microhardness of pure polycrystalline nickel with Ti-DIBM and CrN-DIBM is improved. It was found that the fatigue life of all Ti-DIBM specimens are lower than that of untreated ones in load unload tensile fatigue under stress-controlled condition. That is attributed to it that fatigue cycle stress leads the surface layers to crack and fatigue cracks are accelerated to initiate in many places.
页数70
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17473
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
陈自力. 动态离子束混合对金属腐蚀和疲劳行为的影响[D]. 中国科学院金属研究所. 中国科学院金属研究所,1990.
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