Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides

doi:10.1021/acs.nanolett.2c04972

IMR OpenIR

	Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides
	Jiang, Ru-Jian 1,2; Cao, Yi 1,2; Geng, Wan-Rong 3; Zhu, Mei-Xiong 1,2; Tang, Yun-Long 1; Zhu, Yin-Lian 3; Wang, Yujia 1; Gong, Fenghui 1,2; Liu, Su-Zhen 1,2; Chen, Yu-Ting 1,2; Liu, Jiaqi 1,2; Liu, Nan 1,2; Wang, Jing-Hui 1,2; Lv, Xiao-Dong 1,2; Chen, Shuang-Jie 1,2; Ma, Xiu-Liang 3
通讯作者	Tang, Yun-Long(yltang@imr.ac.cn) ; Zhu, Yin-Lian(zhuyinlian@sslab.org.cn)
	2023-02-01
发表期刊	NANO LETTERS
ISSN	1530-6984
页码	8
摘要	Antiferroelectrics characterized by voltage-driven reversible transitions between antiparallel and parallel polarity are promising for cutting-edge electronic and electrical power applications. Wide-ranging explorations revealing the macroscopic performances and microstructural characteristics of typical antiferroelectric systems have been conducted. However, the underlying mechanism has not yet been fully unraveled, which depends largely on the atomistic processes. Herein, based on atomic-resolution transmission electron microscopy, the deterministic phase transition pathway along with the underlying lattice-by-lattice details in lead zirconate thin films was elucidated. Specifically, we identified a new type of ferrielectric-like dipole configuration with both angular and amplitude modulations, which plays the role of a precursor for a subsequent antiferroelectric to ferroelectric transformation. With the participation of the ferrielectric-like phase, the phase transition pathways driven by the phase boundary have been revealed. We provide new insights into the consecutive phase transformation in low-dimensional lead zirconate, which thus would promote potential antiferroelectric-based multifunctional devices.
关键词	antiferroelectric lead zirconate consecutive phase transformation short-period phase scanning transmission electron microscopy
资助者	National Natural Science Foundation of China ; Key Research Program of Frontier Sciences CAS ; Shenyang National Laboratory for Materials Science ; Scientific Instrument Developing Project of CAS ; Youth Innovation Promotion Association CAS ; Guangdong Basic and Applied Basic Research Foundation ; China Postdoctoral Science Foundation
DOI	10.1021/acs.nanolett.2c04972
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51971223] ; National Natural Science Foundation of China[51922100] ; National Natural Science Foundation of China[52122101] ; Key Research Program of Frontier Sciences CAS[QYZDJ-SSW-JSC010] ; Shenyang National Laboratory for Materials Science[L2019R06] ; Shenyang National Laboratory for Materials Science[L2019R08] ; Shenyang National Laboratory for Materials Science[L2019F01] ; Shenyang National Laboratory for Materials Science[L2019F13] ; Scientific Instrument Developing Project of CAS[YJKYYQ20200066] ; Youth Innovation Promotion Association CAS[Y202048] ; Youth Innovation Promotion Association CAS[2021187] ; Guangdong Basic and Applied Basic Research Foundation[2021A1515110291] ; China Postdoctoral Science Foundation[2022T150690]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号	WOS:000927041400001
出版者	AMER CHEMICAL SOC
引用统计	被引频次：25[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/175131
专题	中国科学院金属研究所
通讯作者	Tang, Yun-Long; Zhu, Yin-Lian
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 3.Bay Area Ctr Electron Microscopy, Songshan Lake Mat Lab, Dongguan 523808, Guangdong, Peoples R China
推荐引用方式 GB/T 7714	Jiang, Ru-Jian,Cao, Yi,Geng, Wan-Rong,et al. Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides[J]. NANO LETTERS,2023:8.
APA	Jiang, Ru-Jian.,Cao, Yi.,Geng, Wan-Rong.,Zhu, Mei-Xiong.,Tang, Yun-Long.,...&Ma, Xiu-Liang.(2023).Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides.NANO LETTERS,8.
MLA	Jiang, Ru-Jian,et al."Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides".NANO LETTERS (2023):8.