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喷吹金属氧化物弥散强化电热合金性能的研究
周丽华
学位类型硕士
导师吴平森
1991
学位授予单位中国科学院金属研究所
学位授予地点中国科学院金属研究所
摘要本文采用向熔融钢液喷吹金属氧化物的喷吹弥散法,得到了弥散强化的Fe-Cr-Al抗氧化合金,以研究金属氧化物对高温晶粒长大、强韧性、冲击断口、高温抗氧化性能和高温使用寿命以及FeCrAl在高温氧化过程中合金力学性能的影响。结果表明,金属氧化物显著降低晶粒的高温长大倾向,这种氧化物粒子对晶界的阻碍作用随着温度的升高而愈加强烈。FeCrAl喷吹金属氧化物后,强韧性明显提高,其中屈服强度提高了167-178MPa,断裂强度提高了129-145MPa冲击韧性提高了2.62-5.19J/cm~2,这可以认为与金属氧化物阻碍位错的运动和增值有关。金属氧化物改善钢的断口形态,未喷吹样品为解理状断口,喷吹氧化物后变为解理与韧窝的混合状断口。本文对Fe-Cr-Al, Fe-Cr-Al-CeO_2,Fe-Cr-Al-ZrO_2三种合金进行了1100 ℃恒温氧化和1250 ℃快速寿命测试的对比实验,并对氧化膜进行扫描电镜电子探针、X射线分析观察。研究发现:金属氧化物降低了氧化速率,其氧化动力学符合抛物线规律。金属氧化物对氧化层相组成没有影响,但改变了氧化膜的分层结构,显著改善了氧化膜的粘附性和致密性,抑制氧化膜与基体间空洞的产生,初步认为金属氧化物能够抑制铝离子向氧化层的扩散,消除了破坏氧化层粘附性和致密性的因素,使氧化层与合金基体产生牢固的结合,寿命试验表明,金属氧化物大幅度提高快速寿命,金属氧化物的加入,使得其寿命未喷吹样品分别提高了86.2%和66.6%,而且金属氧化物微粉使寿命终了时的延伸率分别降低26.9%和31.1%。金属氧化物显著抑制和减缓FeCrAl合金高温氧化过程中力学性能的下降趋势和幅度,这对提高FeCrAl高温使用寿命具有重要意义。
其他摘要A dispersion-strengthening Fe-Cr-Al oxidation-resisting alloy has been made by means of spray-dispersion method which oxide particles are sprayed into molten steel. The oxide particle's effection upon crystal growth at high temperature, tensile strength and toughness, impact fracture shape, high temperature oxidation as well as mechanical properties at high temperature, have been studied. The results indicate that the oxide particles are effective in preventing the trend of the crystal growth at high temperature, and this action that the oxides obstruct the movement of the grain boundaries becomes more striking at higher temperature. There is also a rise in strength and toughness of Fe-Cr-Al alloy with oxide particles and that σ_(0.2) and σ_b increase in the range of 167-178MPa and 129-146MPa, respectively, and a_k increases in the range of 2.62-5.29J/cm~2, this may be considered to the oxide particles preventing the movement and prolifiration of dislocations. Oxides have changed the fracture shapes, the alloy with spraying oxides shows cleavage and ductile dimple cracking and cleavage fracture without oxides. The accelerated oxidation at 1100 ℃ and the rapid heating life test at 1250 ℃ of three alloys: (A) Fe-25Cr-5Al (B) Fe-25Cr-5Al-CeO_2 (C) Fe-25Cr-5Al-ZrO_2, have been examined, and the oxide scales have been observed by SEM. EPMA and X-ray diffraction. It is shown that oxides contribute to a decrease of oxidation rate of the accelerated oxidation which oxidation kinetics conforms to parabolic. Oxides have no infulence upon the phases of the scale but have changed the multi-layer structure of it, exerted correspondingly good influence up the adhesivity and density of the scale and given a control over the presence of the cavities at the scale/substrate interface. Such may be concluded that oxides prevent Al ions from diffusing in the scale and eliminate the facts that destroy the adhesivity and density of the scale and give it a tight adherency to the substrate. The rapid heating life test shows: the oxides remarkably increase the rapid heating life, the addition of oxides makes the life above 86.2% and 66.7% comparision with no spray-alloy, respectively, and the total percentage elongation at the end of test decreases to greater extent. The oxides are found to exert notably good influence up the mechanical properties of the Fe-Cr-Al alloy at high temperature oxidation, such may be very important to increase the heating life of Fe-Cr-Alalloy.
页数64
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17534
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
周丽华. 喷吹金属氧化物弥散强化电热合金性能的研究[D]. 中国科学院金属研究所. 中国科学院金属研究所,1991.
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