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BFe30-1-1铜合金在人工海水中的冲刷腐蚀行为及防护对策研究
杨帆
学位类型硕士
导师姚治铭
1998
学位授予单位中国科学院金属腐蚀与防护研究所
学位授予地点中国科学院金属腐蚀与防护研究所
关键词冲刷腐蚀 Bfe30-1-1 人工海水 石英砂
摘要本文采用旋转圆柱式冲刷腐蚀试验装置通过失重测量、电化学测试(包括交流阻抗、线性极化等)以及SEM、EDX分析等方法研究了BFe30-1-1在单相和含砂的人工海水中的冲刷腐蚀行为以及苯并三氮党代会对该材料冲刷腐的抑制作用。在单相的人工海水中,由失重和线性极化测量结果经计算得出该材料发生冲刷腐蚀反应的电子转移数略大于1,线性极化常数(B)随流速的增加而增加的考极化测量结果表明,流速小于2m/s时材料表现出局部腐蚀敏感性而流速高于2m/s时材料表面不存在完整的腐蚀产物膜;交流阻抗测量结果表明,流速低于2m/s时冲刷腐蚀受扩散过程控制。此外,根据扫描电镜观察,介质流速低于2m/s 时,材料的冲刷腐蚀在试样的轴线方向上呈现出明显的波浪状,而高流速下这种方向性消失。以上试验结果均表明,BFe30-1-1在单相人工海水冲刷腐蚀的临界速度为2m/s。在含砂的人工海水中材料冲刷腐蚀失重和交流阻抗测量结果表明,含砂量大于1%时砂的冲刷对材料腐蚀的促进作用达到了极限,冲刷腐蚀形貌呈溃疡状。缓蚀剂BTA添加于人工海水后,能明显抑制该材料的冲刷腐蚀过程。在流动的人工海水中其作用效果优于静态情况,且对材料在高含砂量的人工海水中冲刷腐蚀有较好的抑制作用,这归因于BTA与材料表面的强配位作用抑制了冲刷腐蚀过程的腐蚀分量和腐蚀对冲刷的促进作用。
其他摘要In this paper, the erosion-corrosion behaviours of BFe30-1-1 in artificial sea water with an without addition of sand have been studied by rotating cylinders erosion-corrosion testing apparatus. The methods adopted in this study include weight loss test, electrochemical measurement such as electrochemical impedance spectrum(EIS), cyclic linear polarization, SEM, EDX, In addition, the inhibition effect of BTA on the erosion-corrosion of BFe30-1-1 has been investigated. In single phase artificial sea water, the transfer electron number of BFe30-1-1 during the course of erosion nd corrosion was calculated to be nearly one. The linear polarization constant(B) increased with increasing fluid velocity. The results obtained from cyclic polarization measurement showed that BFe30-1-1 has a sensitivity of local corrosion for fluid velocity less than 2m/s, however, the sensitivity disappeared for fluid velocity more than 2m/s. According to EIS measurement results, the erosion-corrosion of BFe30-1-1 was controlled by diffusion when fluid velocity was below 2m/s. Furthermore, i can be seen from the photographs of SEM that there exit many waves in axis direction on metal surface for low fluid velocity (<2m/s), however, the waves in same direction can not be found for high fluid velocity(>2m/s). On the basis of above experimental results, it is concluded that there is an experimental results, it concluded that there is a critical velocity of 2m/s for erosion and corrosion of BFe30-1-1 in artificial sea water. In sand containing artificial the water, the results of weight loss test and EIS measurement showed that the action of corrosion on erosion approached a limit when the sand content was higher than 1%, at this time the metal surface had an ulcer morphology. The inhibitor BTA can impress the erosion and corrosion of BFe30-1-1 greatly, especially in nonstatic artificial sea water. BTA still has a good inhibition performance for BFe30-1-1 in the solution with high sand content. All of these can be attributed to the strong interaction between BTA and BFe30-1-1, which reduces the corrosion of BFe30-1-1 and the accelerated action of corrosion on erosion.
页数58
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17641
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
杨帆. BFe30-1-1铜合金在人工海水中的冲刷腐蚀行为及防护对策研究[D]. 中国科学院金属腐蚀与防护研究所. 中国科学院金属腐蚀与防护研究所,1998.
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