Tailoring of electromagnetic properties of arc-produced carbon-coated FeNi alloy nanocapsules for highly efficient microwave absorption | |
Qu, Xinghao1; Javid, Muhammad2; Li, Xiyang1; Huang, Feirong1; Li, Pu3; Duan, Yuping4; Zhang, Zhidong5; Zhang, Xuefeng2; Dong, Xinglong1 | |
Corresponding Author | Dong, Xinglong(dongxl@dlut.edu.cn) |
2023-12-01 | |
Source Publication | DIAMOND AND RELATED MATERIALS
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ISSN | 0925-9635 |
Volume | 140Pages:11 |
Abstract | Due to the growing harm of electromagnetic radiation, it is extremely urgent to develop high-efficiency microwave absorbers with tunable electromagnetic properties. Herein, a simple strategy for synthesizing heteroatoms (sulfur) doped carbon-coated FeNi alloy nanocapsules (FeNi@C(Sx) NCs) by DC arc-discharge plasma was demonstrated. The hetero-interface between the FeNi alloy core and the graphitic shell induce interfacial polarization was found. Meantime, many defects produced by substitutional sulfur atoms in the graphitic shell facilitated dipole polarization and conduction loss. Besides, the multiple magnetic resonance produced by FeNi magnetic alloys worked together to optimize impedance matching. The excellent microwave absorption performance was attributed to the core-shell structure, dipole and interface polarizations, as well as favorable impedance matching. Importantly, the first-principles calculation was applied to prove the charge transfer and polarization process. The minimum reflection loss (RL) can reach up to -50.3 dB at a thickness of 1.6 mm. |
Keyword | FeNi alloy nanocapsules Arc-discharge plasma Substitutional sulfur atoms Interfacial polarization Impedance matchings |
Funding Organization | National Natural Science Foundation of China |
DOI | 10.1016/j.diamond.2023.110487 |
Indexed By | SCI |
Language | 英语 |
Funding Project | National Natural Science Foundation of China[51331006] ; National Natural Science Foundation of China[U1908220] |
WOS Research Area | Materials Science ; Physics |
WOS Subject | Materials Science, Multidisciplinary ; Materials Science, Coatings & Films ; Physics, Applied ; Physics, Condensed Matter |
WOS ID | WOS:001094963400001 |
Publisher | ELSEVIER SCIENCE SA |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/177594 |
Collection | 中国科学院金属研究所 |
Corresponding Author | Dong, Xinglong |
Affiliation | 1.Dalian Univ Technol, Sch Mat Sci & Engn, Key Lab Mat Modificat Laser Ion & Electron Beams, Dalian 116023, Peoples R China 2.Hangzhou Dianzi Univ, Inst Adv Magnet Mat, Coll Mat & Environm Engn, Hangzhou 310012, Peoples R China 3.China United Test & Certificat Co LTD, Gen Res Inst Nonferrous Met, Beijing 100088, Peoples R China 4.Dalian Univ Technol, Sch Mat Sci & Engn, Key Lab Solidifcat Control & Digital Preparat Tech, Dalian 116085, Peoples R China 5.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110015, Liaoning, Peoples R China |
Recommended Citation GB/T 7714 | Qu, Xinghao,Javid, Muhammad,Li, Xiyang,et al. Tailoring of electromagnetic properties of arc-produced carbon-coated FeNi alloy nanocapsules for highly efficient microwave absorption[J]. DIAMOND AND RELATED MATERIALS,2023,140:11. |
APA | Qu, Xinghao.,Javid, Muhammad.,Li, Xiyang.,Huang, Feirong.,Li, Pu.,...&Dong, Xinglong.(2023).Tailoring of electromagnetic properties of arc-produced carbon-coated FeNi alloy nanocapsules for highly efficient microwave absorption.DIAMOND AND RELATED MATERIALS,140,11. |
MLA | Qu, Xinghao,et al."Tailoring of electromagnetic properties of arc-produced carbon-coated FeNi alloy nanocapsules for highly efficient microwave absorption".DIAMOND AND RELATED MATERIALS 140(2023):11. |
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