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Fabrication of Oriented MOF-Based Mixed Matrix Membrane via Ion-Induced Synchronous Synthesis
Zhang, Bing1; Dai, Xueya2; Wei, Nini3,4; Cui, Xingchen1; Fan, Fuqiang1; Zhang, Jidong5; Zhang, Daliang3,4; Meng, Fanbao1; Qi, Wei2; Fu, Yu1
通讯作者Meng, Fanbao(mengfb@mail.neu.edu.cn) ; Qi, Wei(wqi@imr.ac.cn) ; Fu, Yu(fuyu@mail.neu.edu.cn)
2023-11-03
发表期刊SMALL
ISSN1613-6810
页码8
摘要Developing a facile strategy for constructing oriented mixed matrix membranes (MMMs) with uniformly dispersed and high-loading metal-organic frameworks (MOFs) is a crucial scientific challenge in probing the enhanced capability and potential applications of MOF-polymer MMMs. Herein, a novel synchronous synthetic method for constructing oriented CuBDC/poly(m-phenylenediamine) (CuBDC/PmPD) MMM with uniform MOF dispersion at high loading at the air-solution interface via the dual function of metal ions is reported. The resulting MMM exhibits excellent separation performance in ion sieving and seawater desalination due to the structural integrity of the proposed membrane and the highly interconnected channels created through the oriented distribution of MOF in a polymer matrix. Such a cutting-edge approach may provide promising insights into the development of advanced MMMs with optimized structure and superior performances. A novel ion-induced synchronous synthesis strategy is developed for the facile preparation of oriented metal -organic framework (MOF)-polymer mixed matrix membrane (MMM) with uniform dispersion. The synthesized MMM possesses favorable structural integrity and shortened diffusion paths created through the oriented distribution of MOF in a polymer matrix, which exhibits excellent separation performance in ion sieving and seawater desalination.image
关键词ion screening ion-induced synchronous synthesis metal-organic frameworks mixed matrix membrane solar steam evaporation
资助者This work was financially supported by the National Natural Science Foundation of China (22175030) and the Open Project of State Key Laboratory of Supramolecular Structure and Materials (sklssm 202306). Special thanks are due to the instrument from the Ana ; National Natural Science Foundation of China ; Open Project of State Key Laboratory of Supramolecular Structure and Materials
DOI10.1002/smll.202305688
收录类别SCI
语种英语
资助项目This work was financially supported by the National Natural Science Foundation of China (22175030) and the Open Project of State Key Laboratory of Supramolecular Structure and Materials (sklssm 202306). Special thanks are due to the instrument from the Ana[22175030] ; National Natural Science Foundation of China[sklssm 202306] ; Open Project of State Key Laboratory of Supramolecular Structure and Materials
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:001092534100001
出版者WILEY-V C H VERLAG GMBH
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/177741
专题中国科学院金属研究所
通讯作者Meng, Fanbao; Qi, Wei; Fu, Yu
作者单位1.Northeastern Univ, Coll Sci, Dept Chem, Shenyang 110819, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
3.Chongqing Univ, Inst Adv Interdisciplinary Studies, Multiscale Porous Mat Ctr, Chongqing 400044, Peoples R China
4.Chongqing Univ, Sch Chem & Chem Engn, Chongqing 400044, Peoples R China
5.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China
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GB/T 7714
Zhang, Bing,Dai, Xueya,Wei, Nini,et al. Fabrication of Oriented MOF-Based Mixed Matrix Membrane via Ion-Induced Synchronous Synthesis[J]. SMALL,2023:8.
APA Zhang, Bing.,Dai, Xueya.,Wei, Nini.,Cui, Xingchen.,Fan, Fuqiang.,...&Fu, Yu.(2023).Fabrication of Oriented MOF-Based Mixed Matrix Membrane via Ion-Induced Synchronous Synthesis.SMALL,8.
MLA Zhang, Bing,et al."Fabrication of Oriented MOF-Based Mixed Matrix Membrane via Ion-Induced Synchronous Synthesis".SMALL (2023):8.
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