Fundamentals, status and challenges of direct recycling technologies for lithium ion batteries

doi:10.1039/d3cs00254c

IMR OpenIR

	Fundamentals, status and challenges of direct recycling technologies for lithium ion batteries
	Ji, Haocheng 1,2; Wang, Junxiong 1,2,3; Ma, Jun 1,2; Cheng, Hui-Ming 4,5,6; Zhou, Guangmin 1,2
通讯作者	Cheng, Hui-Ming(cheng@imr.ac.cn) ; Zhou, Guangmin(guangminzhou@sz.tsinghua.edu.cn)
	2023-10-27
发表期刊	CHEMICAL SOCIETY REVIEWS
ISSN	0306-0012
页码	51
摘要	Advancement in energy storage technologies is closely related to social development. However, a significant conflict has arisen between the explosive growth in battery demand and resource availability. Facing the upcoming large-scale disposal problem of spent lithium-ion batteries (LIBs), their recycling technology development has become key. Emerging direct recycling has attracted widespread attention in recent years because it aims to 'repair' the battery materials, rather than break them down and extract valuable products from their components. To achieve this goal, a profound understanding of the failure mechanisms of spent LIB electrode materials is essential. This review summarizes the failure mechanisms of LIB cathode and anode materials and the direct recycling strategies developed. We systematically explore the correlation between the failure mechanism and the required repair process to achieve efficient and even upcycling of spent LIB electrode materials. Furthermore, we systematically introduce advanced in situ characterization techniques that can be utilized for investigating direct recycling processes. We then compare different direct recycling strategies, focussing on their respective advantages and disadvantages and their applicability to different materials. It is our belief that this review will offer valuable guidelines for the design and selection of LIB direct recycling methods in future endeavors. Finally, the opportunities and challenges for the future of battery direct recycling technology are discussed, paving the way for its further development. Unlike conventional recycling methods that focus on 'extraction', direct recycling aims for 'repair', which necessitates selecting and designing a recycling strategy based on the failure mechanisms of the spent lithium ion battery materials.
资助者	G. Z. appreciates support from the Joint Funds of the National Natural Science Foundation of China (U21A20174), Guangdong Innovative and Entrepreneurial Research Team Program (2021ZT09L197), Shenzhen Science and Technology Program (KQTD20210811090112002), ; Joint Funds of the National Natural Science Foundation of China ; Guangdong Innovative and Entrepreneurial Research Team Program ; Shenzhen Science and Technology Program ; Interdisciplinary Research and Innovation Fund of Tsinghua Shenzhen International Graduate School ; Tsinghua Shenzhen International Graduate School-Shenzhen Pengrui Young Faculty Program of Shenzhen Pengrui Foundation
DOI	10.1039/d3cs00254c
收录类别	SCI
语种	英语
资助项目	G. Z. appreciates support from the Joint Funds of the National Natural Science Foundation of China (U21A20174), Guangdong Innovative and Entrepreneurial Research Team Program (2021ZT09L197), Shenzhen Science and Technology Program (KQTD20210811090112002),[U21A20174] ; Joint Funds of the National Natural Science Foundation of China[2021ZT09L197] ; Guangdong Innovative and Entrepreneurial Research Team Program[KQTD20210811090112002] ; Shenzhen Science and Technology Program ; Interdisciplinary Research and Innovation Fund of Tsinghua Shenzhen International Graduate School[SZPR2023007] ; Tsinghua Shenzhen International Graduate School-Shenzhen Pengrui Young Faculty Program of Shenzhen Pengrui Foundation
WOS研究方向	Chemistry
WOS类目	Chemistry, Multidisciplinary
WOS记录号	WOS:001090595200001
出版者	ROYAL SOC CHEMISTRY
引用统计	被引频次：38[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/177816
专题	中国科学院金属研究所
通讯作者	Cheng, Hui-Ming; Zhou, Guangmin
作者单位	1.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China 2.Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China 3.Shanghai Jiao Tong Univ, Frontiers Sci Ctr Transformat Mol, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China 4.Chinese Acad Sci, Fac Mat Sci & Energy Engn, Shenzhen 518055, Peoples R China 5.Chinese Acad Sci, Inst Technol Carbon Neutral, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China 6.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Ji, Haocheng,Wang, Junxiong,Ma, Jun,et al. Fundamentals, status and challenges of direct recycling technologies for lithium ion batteries[J]. CHEMICAL SOCIETY REVIEWS,2023:51.
APA	Ji, Haocheng,Wang, Junxiong,Ma, Jun,Cheng, Hui-Ming,&Zhou, Guangmin.(2023).Fundamentals, status and challenges of direct recycling technologies for lithium ion batteries.CHEMICAL SOCIETY REVIEWS,51.
MLA	Ji, Haocheng,et al."Fundamentals, status and challenges of direct recycling technologies for lithium ion batteries".CHEMICAL SOCIETY REVIEWS (2023):51.