Tannic acid coated single-wall carbon nanotube membranes for the recovery of Au from trace-level solutions | |
Wang, Chunmei1,2,3; Hou, Peng-Xiang1,3; Zhao, Yiming1,3; Shi, Chao1; Zhang, Jiangang1,3; Wu, An-Ping1; Liu, Chang1,3; Cheng, Hui-Ming1,4 | |
通讯作者 | Hou, Peng-Xiang(pxhou@imr.ac.cn) ; Liu, Chang(cliu@imr.ac.cn) |
2023-06-27 | |
发表期刊 | NANO RESEARCH
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ISSN | 1998-0124 |
页码 | 8 |
摘要 | The efficient recovery of gold from industrial sewage is important for saving precious metals and remains a big challenge. We report the extraction of gold ions from a trace-level aqueous solution using a tannic acid (TA) coated single-wall carbon nanotube (SWCNT) film. The TA has many redox ligands that efficiently adsorb Au(III) from the solution and reduce them to Au particles. The interwoven SWCNTs not only act as a framework to improve the mechanical stability of the hybrid membrane, but also provide abundant paths for H2O transport, and facilitate the full exposure of the TA. As a result, the hybrid membrane has an excellent ability to capture gold ions from solution with a high flux of 157 L/(m(2)center dot h center dot bar), and an ultra-high adsorption capacity of 2095 mg/g from solutions with an extremely low gold concentration of 20 ppm. The adsorbed gold ions are reduced to Au particles, which can be easily collected by oxidation. The recovered Au nanoparticles on the TA-SWCNT hybrid film had a remarkable surface-enhanced Raman scattering effect that enabled the sensitive detection of rhodamine 6G. |
关键词 | carbon nanotube tannic acid membrane Au recovery redox reaction |
资助者 | National Natural Science Foundation of China ; Liaoning Revitalization Talents Program ; Basic Research Project of the Natural Science Foundation of Shandong Province, China |
DOI | 10.1007/s12274-023-5803-y |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China[52188101] ; National Natural Science Foundation of China[52130209] ; National Natural Science Foundation of China[52072375] ; National Natural Science Foundation of China[51872293] ; Liaoning Revitalization Talents Program[XLYC2002037] ; Basic Research Project of the Natural Science Foundation of Shandong Province, China[ZR2019ZD49] |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
WOS类目 | Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied |
WOS记录号 | WOS:001020364300002 |
出版者 | TSINGHUA UNIV PRESS |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/178544 |
专题 | 中国科学院金属研究所 |
通讯作者 | Hou, Peng-Xiang; Liu, Chang |
作者单位 | 1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Shenyang Univ Chem Technol, Anal & Test Ctr, Shenyang 110142, Peoples R China 3.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 4.Chinese Acad Sci, Inst Technol Carbon Neutral, Shenzhen Inst Adv Technol, Sch Mat Sci & Engn, Shenzhen 518055, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Chunmei,Hou, Peng-Xiang,Zhao, Yiming,et al. Tannic acid coated single-wall carbon nanotube membranes for the recovery of Au from trace-level solutions[J]. NANO RESEARCH,2023:8. |
APA | Wang, Chunmei.,Hou, Peng-Xiang.,Zhao, Yiming.,Shi, Chao.,Zhang, Jiangang.,...&Cheng, Hui-Ming.(2023).Tannic acid coated single-wall carbon nanotube membranes for the recovery of Au from trace-level solutions.NANO RESEARCH,8. |
MLA | Wang, Chunmei,et al."Tannic acid coated single-wall carbon nanotube membranes for the recovery of Au from trace-level solutions".NANO RESEARCH (2023):8. |
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