Enrichment of Large-Diameter Semiconducting Single-Walled Carbon Nanotubes by Conjugated Polymer-Assisted Separation

doi:10.3390/nano13132001

IMR OpenIR

	Enrichment of Large-Diameter Semiconducting Single-Walled Carbon Nanotubes by Conjugated Polymer-Assisted Separation
	Xie, Piao 1; Sun, Yun 1; Chen, Chao 1; Guo, Shu-Yu 1; Zhao, Yiming 1; Jiao, Xinyu 1; Hou, Peng-Xiang 1; Liu, Chang 1; Cheng, Hui-Ming 1,2
通讯作者	Hou, Peng-Xiang(pxhou@imr.ac.cn) ; Liu, Chang(cliu@imr.ac.cn)
	2023-07-01
发表期刊	NANOMATERIALS
卷号	13 期号:13 页码:9
摘要	Semiconducting single-walled carbon nanotubes (s-SWCNTs) with large diameters are highly desired in the construction of high performance optoelectronic devices. However, it is difficult to selectively prepare large-diameter s-SWCNTs since their structure and chemical stability are quite similar with their metallic counterparts. In this work, we use SWCNTs with large diameter as a raw material, conjugated polymer of regioregular poly-(3-dodecylthiophene) (rr-P3DDT) with long side chain as a wrapping agent to selectively separate large-diameter s-SWCNTs. It is found that s-SWCNTs with a diameter of similar to 1.9 nm are effectively enriched, which shows a clean surface. By using the sorted s-SWCNTs as a channel material, we constructed thin-film transistors showing charge-carrier mobilities higher than 10 cm(2) V-1 s(-1) and on/off ratios higher than 10(3).
关键词	semiconducting single-walled carbon nanotubes disperse thin-film transistors
资助者	Ministry of Science and Technology of China ; National Natural Science Foundation of China ; Liaoning Revitalization Talents Program ; Basic Research Project of Natural Science Foundation of Shandong Province, China
DOI	10.3390/nano13132001
收录类别	SCI
语种	英语
资助项目	Ministry of Science and Technology of China[2022YFA1203302] ; National Natural Science Foundation of China[52130209] ; National Natural Science Foundation of China[52188101] ; National Natural Science Foundation of China[52072375] ; Liaoning Revitalization Talents Program[XLYC2002037] ; Basic Research Project of Natural Science Foundation of Shandong Province, China[ZR2019ZD49]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目	Chemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号	WOS:001030260700001
出版者	MDPI
引用统计	被引频次：2[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/178655
专题	中国科学院金属研究所
通讯作者	Hou, Peng-Xiang; Liu, Chang
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Chinese Acad Sci, Inst Technol Carbon Neutral, Shenzhen Inst Adv Technol, Fac Mat Sci & Engn, Shenzhen 518055, Peoples R China
推荐引用方式 GB/T 7714	Xie, Piao,Sun, Yun,Chen, Chao,et al. Enrichment of Large-Diameter Semiconducting Single-Walled Carbon Nanotubes by Conjugated Polymer-Assisted Separation[J]. NANOMATERIALS,2023,13(13):9.
APA	Xie, Piao.,Sun, Yun.,Chen, Chao.,Guo, Shu-Yu.,Zhao, Yiming.,...&Cheng, Hui-Ming.(2023).Enrichment of Large-Diameter Semiconducting Single-Walled Carbon Nanotubes by Conjugated Polymer-Assisted Separation.NANOMATERIALS,13(13),9.
MLA	Xie, Piao,et al."Enrichment of Large-Diameter Semiconducting Single-Walled Carbon Nanotubes by Conjugated Polymer-Assisted Separation".NANOMATERIALS 13.13(2023):9.