Wear-resistant Ag-MAX phase 3D interpenetrating-phase composites: Processing, structure, and properties | |
Guo, Yu1,2; Xie, Xi1; Liu, Zengqian1,2; Zhuo, Longchao3; Zhang, Jian1,4,5; Wang, Shaogang5; Duan, Qiqiang1; Jia, Qing1,2; Xu, Dake4,5; Xue, Weihai1; Duan, Deli1; Berto, Filippo6; Zhang, Zhefeng1,2; Yang, Rui1,2 | |
通讯作者 | Liu, Zengqian(zengqianliu@imr.ac.cn) ; Zhuo, Longchao(zhuolongchao@xaut.edu.cn) ; Zhang, Zhefeng(zhfzhang@imr.ac.cn) |
2023-08-29 | |
发表期刊 | NANO RESEARCH
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ISSN | 1998-0124 |
页码 | 14 |
摘要 | Electrical contact materials are generally Ag- or Cu-based composites and play a critical role in ensuring the reliability and efficiency of electrical equipments and electronic instruments. The MAX (M is an early transition metal, A is an element from III or IV main groups, and X is carbon or/and nitrogen) phase ceramics display a unique combination of properties and may serve as an ideal reinforcement phase for electrical contact materials. The biological materials evolved in nature generally exhibit three-dimensional (3D) interpenetrating-phase architectures, which may offer useful inspiration for the architectural design of electrical contact materials. Here, a series of bi-continuous Ag-Ti3SiC2 MAX phase composites with high ceramic contents exceeding 50 vol.% and having micron- and ultrafine-scaled 3D interpenetrating-phase architectures, wherein both constituents were continuous and mutually interspersed, were exploited by pressureless infiltration of Ag melt into partially sintered Ti3SiC2 scaffolds. The mechanical and electrical properties as well as the friction and wear performance of the composites were investigated and revealed to be closely dependent on the ceramic contents and characteristic structural dimensions. The composites exhibited a good combination of properties with high hardness over 2.3 GPa, high flexural strength exceeding 530 MPa, decent fracture toughness over 10 MPa center dot m1/2, and good wear resistance with low wear rate at an order of 10-5 mm3/(N center dot m), which were much superior compared to the counterparts made by powder metallurgy methods. In particular, the hardness, electrical conductivity, strength, and fracture toughness of the composites demonstrated a simultaneous improvement as the structure was refined from micron- to ultrafine-scales at equivalent ceramic contents. The good combination of properties along with the facile processing route makes the Ag-Ti3SiC2 3D interpenetrating-phase composites appealing for electrical contact applications. |
关键词 | three-dimensional (3D) interpenetrating-phase architecture Ag-MAX (M = early transition metal A = element from III or IV main groups and X = carbon or/and nitrogen) phase composites melt infiltration electrical contact materials mechanical properties wear resistance |
资助者 | The authors are grateful for the financial supports from the National Key Ramp;D Program of China (No. 2020YFA0710404), the National Natural Science Foundation of China (No. 52173269), the KC Wong Education Foundation (No. GJTD-2020-09), the Liaoning Revi ; National Key Ramp;D Program of China ; National Natural Science Foundation of China ; KC Wong Education Foundation ; Liaoning Revitalization Talents Program ; Youth Innovation Promotion Association CAS |
DOI | 10.1007/s12274-023-6015-1 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | The authors are grateful for the financial supports from the National Key Ramp;D Program of China (No. 2020YFA0710404), the National Natural Science Foundation of China (No. 52173269), the KC Wong Education Foundation (No. GJTD-2020-09), the Liaoning Revi[2020YFA0710404] ; National Key Ramp;D Program of China[52173269] ; National Natural Science Foundation of China[GJTD-2020-09] ; KC Wong Education Foundation ; Liaoning Revitalization Talents Program[2019191] ; Youth Innovation Promotion Association CAS |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
WOS类目 | Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied |
WOS记录号 | WOS:001080763000004 |
出版者 | TSINGHUA UNIV PRESS |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/179462 |
专题 | 中国科学院金属研究所 |
通讯作者 | Liu, Zengqian; Zhuo, Longchao; Zhang, Zhefeng |
作者单位 | 1.Chinese Acad Sci, Shi Changxu Innovat Ctr Adv Mat, Inst Met Res, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Peoples R China 3.Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Peoples R China 4.Northeastern Univ, Electrobiomat Inst, Key Lab Anisotropy & Texture Mat, Minist Educ, Shenyang 110819, Peoples R China 5.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 6.Sapienza Univ Roma, Dept Chem Engn Mat Environm, I-00185 Rome, Italy |
推荐引用方式 GB/T 7714 | Guo, Yu,Xie, Xi,Liu, Zengqian,et al. Wear-resistant Ag-MAX phase 3D interpenetrating-phase composites: Processing, structure, and properties[J]. NANO RESEARCH,2023:14. |
APA | Guo, Yu.,Xie, Xi.,Liu, Zengqian.,Zhuo, Longchao.,Zhang, Jian.,...&Yang, Rui.(2023).Wear-resistant Ag-MAX phase 3D interpenetrating-phase composites: Processing, structure, and properties.NANO RESEARCH,14. |
MLA | Guo, Yu,et al."Wear-resistant Ag-MAX phase 3D interpenetrating-phase composites: Processing, structure, and properties".NANO RESEARCH (2023):14. |
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