Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries

doi:10.1002/smll.202410036

IMR OpenIR

	Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries
	Li, Shengwei 1; Das, Pratteek 1; Wang, Xiao 1; Li, Chenyang 1; Wu, Zhong-Shuai 1; Cheng, Hui-Ming 2,3,4
通讯作者	Wu, Zhong-Shuai(wuzs@dicp.ac.cn) ; Cheng, Hui-Ming(hm.cheng@siat.ac.cn)
	2025-01-24
发表期刊	SMALL
ISSN	1613-6810
页码	16
摘要	Aqueous zinc-based batteries (AZBs) are gaining widespread attention owing to their intrinsic safety, relatively low electrode potential, and high theoretical capacity. Transition metal dichalcogenides (TMDs) have convenient 2D ion diffusion channels, so they have been identified as promising host materials for AZBs, but face several key challenges such as the narrow interlayer spacing and the lack of in-deep understanding energy storage mechanisms. This review presents a comprehensive summary and discussion of the intrinsic structure, charge storage mechanisms, and key fabrication strategies of TMD-based cathodes for AZBs. Firstly, the structural features including phase types and electrical properties of TMDs are underscored. Then, the charge storage mechanisms and activation principles in TMDs are elaborated along with the discussions about their influence on electrochemical performance. Afterward, specific attention is focused on the fabrication strategies of high-performance TMD cathodes, including interlayer expansion, defect creation, phase transition, and heteroatom doping. Finally, the key challenges are considered and potential effective strategies are proposed to design high-performance aqueous Zn-TMDs batteries.
关键词	aqueous Zn-based battery cathode fabrication strategy transition metal dichalcogenides
资助者	National Natural Science Foundation of China ; Basic Science Center Project of the National Natural Science Foundation of China ; China National Postdoctoral Program for Innovative Talents ; Natural Science Foundation of Liaoning Province ; DICP ; State Key Laboratory of Catalysis ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy
DOI	10.1002/smll.202410036
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China ; Basic Science Center Project of the National Natural Science Foundation of China[52188101] ; China National Postdoctoral Program for Innovative Talents[BX20240361] ; Natural Science Foundation of Liaoning Province[2024-BSBA-31] ; DICP[DICP I202471] ; State Key Laboratory of Catalysis[2024SKL-A-001] ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy[E412010508] ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy[E411050316] ; [22125903] ; [22439003] ; [22309176] ; [22209173] ; [22409196] ; [W2433043]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号	WOS:001403213800001
出版者	WILEY-V C H VERLAG GMBH
引用统计
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/180450
专题	中国科学院金属研究所
通讯作者	Wu, Zhong-Shuai; Cheng, Hui-Ming
作者单位	1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen Key Lab Energy Mat Carbon Neutral, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 4.Shenzhen Univ Adv Technol, Fac Mat Sci & Energy Engn, Shenzhen 518055, Peoples R China
推荐引用方式 GB/T 7714	Li, Shengwei,Das, Pratteek,Wang, Xiao,et al. Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries[J]. SMALL,2025:16.
APA	Li, Shengwei,Das, Pratteek,Wang, Xiao,Li, Chenyang,Wu, Zhong-Shuai,&Cheng, Hui-Ming.(2025).Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries.SMALL,16.
MLA	Li, Shengwei,et al."Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries".SMALL (2025):16.