Deep-Ultraviolet and Helicity-Dependent Raman Spectroscopy for Carbon Nanotubes and 2D Materials | |
Saito, Riichiro1,2; Hung, Nguyen Tuan3; Yang, Teng4; Huang, Jianqi4; Liu, Hsiang-Lin1; Gulo, Desman Perdamaian1; Han, Shiyi5; Tong, Lianming5 | |
通讯作者 | Saito, Riichiro(rsaito@tohoku.ac.jp) ; Hung, Nguyen Tuan(nguyen.tuan.hung.e4@tohoku.ac.jp) ; Liu, Hsiang-Lin(hliu@ntnu.edu.tw) ; Tong, Lianming(tonglm@pku.edu.cn) |
2024-02-27 | |
发表期刊 | SMALL
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ISSN | 1613-6810 |
页码 | 17 |
摘要 | Recent progress of Raman spectroscopy on carbon nanotubes and 2D materials is reviewed as a topical review. The Raman tensor with complex values is related to the chiral 1D/2D materials without mirror symmetry for the mirror in the propagating direction of light, such as chiral carbon nanotube and black phosphorus. The phenomenon of complex Raman tensor is observed by the asymmetric polar plot of helicity-dependent Raman spectroscopy using incident circularly-polarized lights. First-principles calculations of resonant Raman spectra directly give the complex Raman tensor that explains helicity-dependent Raman spectra and laser-energy-dependent relative intensities of Raman spectra. In deep-ultraviolet (DUV) Raman spectroscopy with 266 nm laser, since the energy of the photon is large compared with the energy gap, the first-order and double resonant Raman processes occur in general k points in the Brillouin zone. First-principles calculation is necessary to understand the DUV Raman spectra and the origin of double-resonance Raman spectra. Asymmetric line shapes appear for the G band of graphene for 266 nm laser and in-plane Raman mode of WS2 for 532 nm laser, while these spectra show symmetric line shapes for other laser excitation. The interference effect on the asymmetric line shape is discussed by fitting the spectra to the Breit-Wigner-Fano line shapes. Recent progress of Raman spectroscopy using deep-ultraviolet light and circularly polarized light and first-principles calculation for single and double resonance Raman spectra. image |
关键词 | deep-ultraviolet Raman spectroscopy helicity-dependent Raman spectra tip-enhanced Raman spectroscopy |
资助者 | JSPS KAKENHI ; JSPS KAKENHI Grant ; Ministry of Education (MOE), Taiwan ; Frontier Research Institute for Interdisciplinary Sciences, Tohoku University ; National Science and Technology Council of Taiwan ; National Natural Science Foundation of China ; National Key R&D Program of China |
DOI | 10.1002/smll.202308558 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | JSPS KAKENHI[JP22H00283] ; JSPS KAKENHI Grant ; Ministry of Education (MOE), Taiwan ; Frontier Research Institute for Interdisciplinary Sciences, Tohoku University[112-2112-M-003-017] ; National Science and Technology Council of Taiwan[52031014] ; National Natural Science Foundation of China[2022YFA1203901] ; National Key R&D Program of China |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
WOS类目 | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
WOS记录号 | WOS:001173797100001 |
出版者 | WILEY-V C H VERLAG GMBH |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/184851 |
专题 | 中国科学院金属研究所 |
通讯作者 | Saito, Riichiro; Hung, Nguyen Tuan; Liu, Hsiang-Lin; Tong, Lianming |
作者单位 | 1.Natl Taiwan Normal Univ, Dept Phys, Taipei 11677, Taiwan 2.Tohoku Univ, Dept Phys, Sendai 9808578, Japan 3.Tohoku Univ, Frontier Res Inst Interdisciplinary Sci, Sendai 9808578, Japan 4.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 5.Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China |
推荐引用方式 GB/T 7714 | Saito, Riichiro,Hung, Nguyen Tuan,Yang, Teng,et al. Deep-Ultraviolet and Helicity-Dependent Raman Spectroscopy for Carbon Nanotubes and 2D Materials[J]. SMALL,2024:17. |
APA | Saito, Riichiro.,Hung, Nguyen Tuan.,Yang, Teng.,Huang, Jianqi.,Liu, Hsiang-Lin.,...&Tong, Lianming.(2024).Deep-Ultraviolet and Helicity-Dependent Raman Spectroscopy for Carbon Nanotubes and 2D Materials.SMALL,17. |
MLA | Saito, Riichiro,et al."Deep-Ultraviolet and Helicity-Dependent Raman Spectroscopy for Carbon Nanotubes and 2D Materials".SMALL (2024):17. |
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