Toward Direct Regeneration of Spent Lithium-Ion Batteries: A Next-Generation Recycling Method

doi:10.1021/acs.chemrev.3c00884

IMR OpenIR

	Toward Direct Regeneration of Spent Lithium-Ion Batteries: A Next-Generation Recycling Method
	Wang, Junxiong 1,2; Ma, Jun 1; Zhuang, Zhaofeng 1; Liang, Zheng 2; Jia, Kai 1,2; Ji, Guanjun 1,2; Zhou, Guangmin 1; Cheng, Hui-Ming 3,4
通讯作者	Liang, Zheng(liangzheng06@sjtu.edu.cn) ; Zhou, Guangmin(guangminzhou@sz.tsinghua.edu.cn) ; Cheng, Hui-Ming(hm.cheng@siat.ac.cn)
	2024-03-01
发表期刊	CHEMICAL REVIEWS
ISSN	0009-2665
卷号	124 期号:5 页码:2839-2887
摘要	The popularity of portable electronic devices and electric vehicles has led to the drastically increasing consumption of lithium-ion batteries recently, raising concerns about the disposal and recycling of spent lithium-ion batteries. However, the recycling rate of lithium-ion batteries worldwide at present is extremely low. Many factors limit the promotion of the battery recycling rate: outdated recycling technology is the most critical one. Existing metallurgy-based recycling methods rely on continuous decomposition and extraction steps with high-temperature roasting/acid leaching processes and many chemical reagents. These methods are tedious with worse economic feasibility, and the recycling products are mostly alloys or salts, which can only be used as precursors. To simplify the process and improve the economic benefits, novel recycling methods are in urgent demand, and direct recycling/regeneration is therefore proposed as a next-generation method. Herein, a comprehensive review of the origin, current status, and prospect of direct recycling methods is provided. We have systematically analyzed current recycling methods and summarized their limitations, pointing out the necessity of developing direct recycling methods. A detailed analysis for discussions of the advantages, limitations, and obstacles is conducted. Guidance for future direct recycling methods toward large-scale industrialization as well as green and efficient recycling systems is also provided.
资助者	National Natural Science Foundation of China
DOI	10.1021/acs.chemrev.3c00884
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China
WOS研究方向	Chemistry
WOS类目	Chemistry, Multidisciplinary
WOS记录号	WOS:001181995600001
出版者	AMER CHEMICAL SOC
引用统计
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/184874
专题	中国科学院金属研究所
通讯作者	Liang, Zheng; Zhou, Guangmin; Cheng, Hui-Ming
作者单位	1.Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China 2.Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Frontiers Sci Ctr Transformat Mol, Shanghai 200240, Peoples R China 3.Chinese Acad Sci, Shenzhen Inst Adv Technol, Fac Mat Sci & Engn, Inst Technol Carbon Neutral, Shenzhen 518055, Peoples R China 4.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Wang, Junxiong,Ma, Jun,Zhuang, Zhaofeng,et al. Toward Direct Regeneration of Spent Lithium-Ion Batteries: A Next-Generation Recycling Method[J]. CHEMICAL REVIEWS,2024,124(5):2839-2887.
APA	Wang, Junxiong.,Ma, Jun.,Zhuang, Zhaofeng.,Liang, Zheng.,Jia, Kai.,...&Cheng, Hui-Ming.(2024).Toward Direct Regeneration of Spent Lithium-Ion Batteries: A Next-Generation Recycling Method.CHEMICAL REVIEWS,124(5),2839-2887.
MLA	Wang, Junxiong,et al."Toward Direct Regeneration of Spent Lithium-Ion Batteries: A Next-Generation Recycling Method".CHEMICAL REVIEWS 124.5(2024):2839-2887.