Status and Prospect of Two-Dimensional Materials in Electrolytes for All-Solid-State Lithium Batteries

doi:10.1021/acsnano.4c00128

IMR OpenIR

	Status and Prospect of Two-Dimensional Materials in Electrolytes for All-Solid-State Lithium Batteries
	Lan, Xuexia 1; Luo, Na 1; Li, Zhen 1; Peng, Jing 1,2,3; Cheng, Hui-Ming 1,2,3,4
通讯作者	Peng, Jing(jing.peng@siat.ac.cn) ; Cheng, Hui-Ming(hm.cheng@siat.ac.cn)
	2024-03-24
发表期刊	ACS NANO
ISSN	1936-0851
卷号	18 期号:13 页码:9285-9310
摘要	Replacing liquid electrolytes and separators in conventional lithium-ion batteries with solid-state electrolytes (SSEs) is an important strategy to ensure both high energy density and high safety. Searching for fast ionic conductors with high electrochemical and chemical stability has been the core of SSE research and applications over the past decades. Based on the atomic-level thickness and infinitely expandable planar structure, numerous two-dimensional materials (2DMs) have been exploited and applied to address the most critical issues of low ionic conductivity of SSEs and lithium dendrite growth in all-solid-state lithium batteries. This review introduces the research process of 2DMs in SSEs, then summarizes the mechanisms and strategies of inert and active 2DMs toward Li+ transport to improve the ionic conductivity and enhance the electrode/SSE interfacial compatibility. More importantly, the main challenges and future directions for the application of 2DMs in SSEs are considered, including the importance of exploring the relationship between the anisotropic structure of 2DMs and Li+ diffusion behavior, the exploitation of more 2DMs, and the significance of in situ characterizations in elucidating the mechanisms of Li+ transport and interfacial reactions. This review aims to provide a comprehensive understanding to facilitate the application of 2DMs in SSEs.
关键词	two-dimensional materials solid-state electrolytes ionic conductivity all-solid-state lithium batteries interface compatibility lithium dendrites stability mechanical properties design strategies
资助者	Science and Technology Foundation of Shenzhen City ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; Science and Technology Foundation of Shenzhen ; Guang Dong Basic and Applied Basic Research Foundation ; China Postdoctoral Science Foundation ; Cross Institute Joint Research Youth Team Project of SIAT
DOI	10.1021/acsnano.4c00128
收录类别	SCI
语种	英语
资助项目	Science and Technology Foundation of Shenzhen City[2022YFB3803400] ; National Key Research and Development Program of China[52188101] ; National Key Research and Development Program of China[22275205] ; National Key Research and Development Program of China[52302332] ; National Natural Science Foundation of China[JCYJ20200109144616617] ; National Natural Science Foundation of China[JCYJ20220818100806014] ; National Natural Science Foundation of China[JCYJ20220530154404010] ; Science and Technology Foundation of Shenzhen[2023B1515020102] ; Guang Dong Basic and Applied Basic Research Foundation[2023M733644] ; Guang Dong Basic and Applied Basic Research Foundation[BX20230398] ; China Postdoctoral Science Foundation[E25427] ; Cross Institute Joint Research Youth Team Project of SIAT
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:001190665600001
出版者	AMER CHEMICAL SOC
引用统计
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/184953
专题	中国科学院金属研究所
通讯作者	Peng, Jing; Cheng, Hui-Ming
作者单位	1.Chinese Acad Sci, Inst Technol Carbon Neutral, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China 2.Shenzhen Inst Adv Technol, Fac Mat Sci & Energy Engn, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen Key Lab Energy Mat Carbon Neutral, Shenzhen 518055, Peoples R China 4.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang, Peoples R China
推荐引用方式 GB/T 7714	Lan, Xuexia,Luo, Na,Li, Zhen,et al. Status and Prospect of Two-Dimensional Materials in Electrolytes for All-Solid-State Lithium Batteries[J]. ACS NANO,2024,18(13):9285-9310.
APA	Lan, Xuexia,Luo, Na,Li, Zhen,Peng, Jing,&Cheng, Hui-Ming.(2024).Status and Prospect of Two-Dimensional Materials in Electrolytes for All-Solid-State Lithium Batteries.ACS NANO,18(13),9285-9310.
MLA	Lan, Xuexia,et al."Status and Prospect of Two-Dimensional Materials in Electrolytes for All-Solid-State Lithium Batteries".ACS NANO 18.13(2024):9285-9310.