Temperature effect on the passivation of a novel Fe-based metallic glass in simulated wet storage environment of spent nuclear fuels

doi:10.1007/s10853-024-10144-2

IMR OpenIR

	Temperature effect on the passivation of a novel Fe-based metallic glass in simulated wet storage environment of spent nuclear fuels
	Huang, Ping 1,2; Zhang, Suode 2; Ren, Yinglei 1; Wang, Debin 2,3; Qiu, Keqiang 1; Wang, Jianqiang 2
通讯作者	Wang, Debin(dbwang18s@imr.ac.cn) ; Qiu, Keqiang(kqqiu@sut.edu.cn) ; Wang, Jianqiang(jqwang@imr.ac.cn)
	2024-09-01
发表期刊	JOURNAL OF MATERIALS SCIENCE
ISSN	0022-2461
卷号	59 期号:34 页码:16274-16291
摘要	The corrosion behavior of a novel Fe57Cr10Mo5Nb2Zr8B18 metallic glass (MG) and BSS in simulated wet storage environment of spent nuclear fuels at different temperatures was studied comparatively by electrochemical techniques. The experimental results indicated that the pitting potentials of MG were significantly higher than that of BSS, and the passive current densities were lower than that of BSS and high-chromium SAM2X5 amorphous steel due to the synergistic effect of Cr and Mo elements. With the temperature elevating from 30 degrees C to 70 degrees C, the passive current densities of metallic glass were increased by about one order of magnitude. The passive current temperature sensitivity for this metallic glass was closely related to the decreased Cr2O3 content, increased donor density and reduced work function of the passive film. This work provides a new insight for developing novel alloys with high corrosion resistance as well as excellent neutron absorption capacity for applications in spent nuclear fuel storage.
资助者	National Natural Science Foundation of China ; Key Research Program of the Chinese Academy of Sciences
DOI	10.1007/s10853-024-10144-2
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[U1908219] ; National Natural Science Foundation of China[52171163] ; Key Research Program of the Chinese Academy of Sciences[ZDRW-CN-2021-2-2]
WOS研究方向	Materials Science
WOS类目	Materials Science, Multidisciplinary
WOS记录号	WOS:001304862400002
出版者	SPRINGER
引用统计	被引频次：1[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/189814
专题	中国科学院金属研究所
通讯作者	Wang, Debin; Qiu, Keqiang; Wang, Jianqiang
作者单位	1.Shenyang Univ Technol, Sch Mat Sci & Engn, Shenyang 110870, Peoples R China 2.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China 3.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Huang, Ping,Zhang, Suode,Ren, Yinglei,et al. Temperature effect on the passivation of a novel Fe-based metallic glass in simulated wet storage environment of spent nuclear fuels[J]. JOURNAL OF MATERIALS SCIENCE,2024,59(34):16274-16291.
APA	Huang, Ping,Zhang, Suode,Ren, Yinglei,Wang, Debin,Qiu, Keqiang,&Wang, Jianqiang.(2024).Temperature effect on the passivation of a novel Fe-based metallic glass in simulated wet storage environment of spent nuclear fuels.JOURNAL OF MATERIALS SCIENCE,59(34),16274-16291.
MLA	Huang, Ping,et al."Temperature effect on the passivation of a novel Fe-based metallic glass in simulated wet storage environment of spent nuclear fuels".JOURNAL OF MATERIALS SCIENCE 59.34(2024):16274-16291.