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Ferromagnetic tendency at the surface of CE-type charge-ordered manganites
S. Dong; R. Yu; S. Yunoki; J. M. Liu; E. Dagotto
2008
Source PublicationPhysical Review B
ISSN1098-0121
Volume78Issue:6
AbstractMost previous investigations have shown that the surface of a ferromagnetic material may have antiferromagnetic tendencies. However, experimentally, the opposite effect has been recently observed-ferromagnetism appears in some nanosized manganites with a composition such that the antiferromagnetic charge-ordered CE state is observed in the bulk. A possible origin is the development of ferromagnetic correlations at the surface of these small systems. To clarify these puzzling experimental observations, we have studied the two-orbital double-exchange model near half doping, n = 0.5, using open boundary conditions to simulate the surface of either bulk or nanosized manganites. Considering the enhancement of surface charge density due to a possible AO termination (A = trivalent/divalent ion composite, O = oxygen), an unexpected surface phase-separated state emerges when the model is studied using Monte Carlo techniques on small clusters. This tendency suppresses the CE charge ordering and produces a weak ferromagnetic signal that could explain the experimental observations.
description.department[dong, shuai; yu, rong; yunoki, seiji; dagotto, elbio] univ tennessee, dept phys & astron, knoxville, tn 37996 usa. [dong, shuai; yu, rong; yunoki, seiji; dagotto, elbio] oak ridge natl lab, mat sci & technol div, oak ridge, tn 37831 usa. [dong, shuai; liu, j. -m.] nanjing univ, nanjing natl lab microstruct, nanjing 210093, peoples r china. [liu, j. -m.] chinese acad sci, int ctr mat phys, shenyang 110016, peoples r china.;dong, s (reprint author), univ tennessee, dept phys & astron, knoxville, tn 37996 usa
KeywordDouble-exchange Model Magnetic-properties Doped Manganites Phase-diagram Low-temperature States La2/3sr1/3mno3 Nanoparticles
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WOS IDWOS:000259264900063
Citation statistics
Cited Times:138[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/32720
Collection中国科学院金属研究所
Recommended Citation
GB/T 7714
S. Dong,R. Yu,S. Yunoki,et al. Ferromagnetic tendency at the surface of CE-type charge-ordered manganites[J]. Physical Review B,2008,78(6).
APA S. Dong,R. Yu,S. Yunoki,J. M. Liu,&E. Dagotto.(2008).Ferromagnetic tendency at the surface of CE-type charge-ordered manganites.Physical Review B,78(6).
MLA S. Dong,et al."Ferromagnetic tendency at the surface of CE-type charge-ordered manganites".Physical Review B 78.6(2008).
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