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The effect of sulfur on the structure of carbon nanotubes produced by a floating catalyst method
W. C. Ren; F. Li; S. Bai; H. M. Cheng
2006
发表期刊Journal of Nanoscience and Nanotechnology
ISSN1533-4880
卷号6期号:5页码:1339-1345
摘要The effect of sulfur on the structures (shell number and diameter distribution) of carbon nanotubes (CNTs) was investigated in detail using high resolution transmission electronic microscopy (HRTEM) and Raman spectroscopy. Single-walled (SWNTs), double-walled (DWNTs), and multi-walled carbon nanotubes (MWNTs) with different diameter distributions were obtained only by increasing the sulfur addition amount with methane as carbon source. A similar structure change was found for ethanol as carbon source with changing the sulfur addition amount. These results indicate that addition of sulfur is necessary to enhance the growth of SWNTs and DWNTs, independent of the carbon source for our method. Based on the growth parameter study, HRTEM observations and kinetic considerations, the role of sulfur in the nucleation and growth of CNTs was discussed.
部门归属chinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china.;cheng, hm (reprint author), chinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china
关键词Carbon Nanotubes Nucleation Growth Mechanism Electron Microscopy Raman Spectroscopy Diameter Distribution Raman-scattering Metal Particles Growth Nanofibers Decomposition Morphology Hydrocarbons Mechanism Methane
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WOS记录号WOS:000238030200019
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被引频次:62[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/34442
专题中国科学院金属研究所
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W. C. Ren,F. Li,S. Bai,et al. The effect of sulfur on the structure of carbon nanotubes produced by a floating catalyst method[J]. Journal of Nanoscience and Nanotechnology,2006,6(5):1339-1345.
APA W. C. Ren,F. Li,S. Bai,&H. M. Cheng.(2006).The effect of sulfur on the structure of carbon nanotubes produced by a floating catalyst method.Journal of Nanoscience and Nanotechnology,6(5),1339-1345.
MLA W. C. Ren,et al."The effect of sulfur on the structure of carbon nanotubes produced by a floating catalyst method".Journal of Nanoscience and Nanotechnology 6.5(2006):1339-1345.
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